Responsive polymer brushes grafted from gold nanoparticles: interaction with surfactant

DOI

We will use SANS to characterize dispersions of gold nanoparticles functionalized with poly(dimethyl aminoethyl methacrylate) brushes grafted from 25 nm gold nanoparticle interfaces by surface-initiated ATRP. We will characterize the response of the polymer layers to pH and at at low pH, where the polymer is cationically charged, to electrolyte concentration. Our main focus however will be to determine the nature of the surfactant aggregates formed in the brushes at concentrations of surfactant that lead to peaks in the surface tension of the dispersions at pH=3 and 10 and also lead to the formation of multilayer structures in equivalent brushes formed at planar interfaces. We will measure under particle-matching contrast, for dispersions bearing hydrogenous pDMAMEA and particle-matching DMAEMA with particle-matching SDS and hydrogenous SDS respectively.

Identifier
DOI https://doi.org/10.5286/ISIS.E.24079886
Metadata Access https://icatisis.esc.rl.ac.uk/oaipmh/request?verb=GetRecord&metadataPrefix=oai_datacite&identifier=oai:icatisis.esc.rl.ac.uk:inv/24079886
Provenance
Creator Dr Simon Titmuss; Mr Haidong Jia
Publisher ISIS Neutron and Muon Source
Publication Year 2013
Rights CC-BY Attribution 4.0 International; https://creativecommons.org/licenses/by/4.0/
OpenAccess true
Contact isisdata(at)stfc.ac.uk
Representation
Resource Type Dataset
Discipline Photon- and Neutron Geosciences
Temporal Coverage Begin 2010-05-01T07:45:00Z
Temporal Coverage End 2010-05-04T08:32:54Z