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Artificial [FeFe]-Hydrogenases and Muon Spectroscopy
Preliminary measurements of [FeFe]-hydrogenase model complexes were made in a previous experiment using EMU (RB 1010177). The results were interpreted in combination with DFT... -
Muon Spin Relaxation and ALC Resonance in Magnetic and non-Magnetic Oxalate S...
Repolarisation and level crossing resonance will be studied for several different oxalate compounds where muon radical states are known to be formed. Such compounds form a... -
Mechanical disorder-induced quantum spin liquid in a two-dimensional triangul...
The quantum spin liquid (QSL) state is one of the possible outcomes of quantum fluctuations advancing magnetic systems into a disordered phase. After more than 30 years of quest... -
Repolarization of Radicals in Liquids
The recovery of the muon polarization in a longitudinal magnetic field has been used to obtain the muon hfcs of organic radicals. In pure benzene there is a single step in the... -
Muon level-crossing resonances as a probe for studying antiferromagnets at pu...
We propose a set of measurements using the HiFi spectrometer in which muon level-crossing resonances are used to probe the internal field inside antiferromagnets in which the... -
Hunting for the low-temperature, low-field magnetization plateau in Tb2Ti2O7
Tb2Ti2O7 is a pyrochlore antiferromagnet that has previously been viewed as a spin liquid. This description fails to describe key features of its physics and more recently the... -
Muonium in rare-earth sesquioxides
We propose to characterize the basic muonium/hydrogen configurations in selected rare-earth sesquioxides with the basic crystallographic structures: neodymium oxide (hexagonal A... -
Models of the [FeFe]-hydrogenase active site: raising the symmetry
The [FeFe]-hydrogenase enzymes are some of the best catalysts know for generating hydrogen. We have an ongoing programme to understand how their chemistry works, and to... -
Muon spin relaxation studies of KTCNQ and related compounds
Potassium tetracyanoquinodimenthane (KTCNQ) undergoes a spin-Peierls (SP) transition at 396K where a transformation from uniform to dimerised TCNQ- molecules in 1D columns... -
RF MuSR in the gas phase: the Search for a Radical State
The main spectroscopic technique for studying radicals in solids and liquids, ESR, cannot usually be used to study radicals of more than 3-5 atoms in the gas phase due to strong... -
Using muons to investigate the excitation spectrum in low-dimensional molecul...
We propose to use longitudinal field muon-spin relaxation to investigate the excitation spectrum of the most successful realizations of one- and two-dimensional antiferromagnets... -
Muon response to changes in the charge distribution of the components of a co...
We plan to confirm that the change in asymmetry on resonance in the ALC spectra seen in the subject complex dielectric during the previous rapid access proposal (RB1900028) is a... -
Unconventional superconductivity in quasi-1D K_2Cr_3As_3 (QLCR)
Metallic systems with one-dimensional chain-like atomic structure can support unusual mechanisms for electron pairing leading to superconductivity. K_2Cr_3As_3 is one of a... -
RF MuSR in the gas phase: The Search for a Radical State (RB920227)
The main spectroscopic technique for studying radicals in solids and liquids, ESR, cannot usually be used to study radicals of more than 3-5 atoms in the gas phase due to strong... -
Muon Spectroscopy Training School
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Muon States in Nanostructured Carbonaceous Materials
This experiment proposes the continuation of a study, initiated at J-PARC, on a new type of activated carbon material, with a pore structure and chemistry "tunable" in a manner... -
Oxygen deficiency in the quantum spin ice Tb2Ti2O7
Tb2Ti2O7 is one of two compounds identified as potential quantum spin ices. As with other oxide pyrochlores the properties depend sensitively on the oxygen content. Most... -
Quantum tunnelling of muonium via radical states in molecular solids
The extreme quantum nature of muons and muonium in condensed matter is the result of having a mass that is nine times lighter than that of a hydrogen atom. While this quantum... -
A second generation 2D antiferromagnet investigated with muons
Low-dimensional quantum magnetism continues to be of great theoretical and experimental interest, as reduced dimensionality supports strong quantum fluctuations which can result... -
Muon level-crossing resonances as a probe for studying antiferromagnets at pu...
We propose a set of measurements using the HiFi spectrometer in which muon level-crossing resonances are used to probe the internal field inside antiferromagnets in which the...
