Multi-catalyst ensembles - aggregation structure and selectivity

DOI

There is exciting potential for SANS to resolve an important problem in homogeneous catalyst chemistry. The Pd-chiral catalyst 1+ below has significant pan-industrial potential applications, being almost unique for having high selectivity in chiral syntheses. Certain solution conditions trigger a remarkable (and as yet unexplained) shift in selectivity: the catalyst is still effective, but it now loses the all-important chiral selectivity. Based on extensive 31P-NMR and trial SANS, this thought to be owing to aggregation/oligmerization to generate (1+)n . The requested beam time will allow this intriguing system to be interrogated in detail, to help explain the unusual properties for design of second generation catalysts which retain chiral activity. The PI is a new user, working in collaboration with Eastoe¿s experienced neutron research team

Identifier
DOI https://doi.org/10.5286/ISIS.E.24083823
Metadata Access https://icatisis.esc.rl.ac.uk/oaipmh/request?verb=GetRecord&metadataPrefix=oai_datacite&identifier=oai:icatisis.esc.rl.ac.uk:inv/24083823
Provenance
Creator Professor Julian Eastoe; Dr Kieran Trickett; Mr Stephen Cummings; Professor Guy Lloyd-Jones; Mr Azmi Mohamed; Mr Rodrigo de Oliveira; Dr Marios Hopkins Hatzopoulos
Publisher ISIS Neutron and Muon Source
Publication Year 2014
Rights CC-BY Attribution 4.0 International; https://creativecommons.org/licenses/by/4.0/
OpenAccess true
Contact isisdata(at)stfc.ac.uk
Representation
Resource Type Dataset
Discipline Photon- and Neutron Geosciences
Temporal Coverage Begin 2011-04-06T10:21:50Z
Temporal Coverage End 2011-04-08T10:30:09Z