Bi0.775Ln0.225O1.5 (Ln = La, Dy) Oxide Ion Conductors: Local Structure, Complex Superstructures and Structural Phase Transitions

DOI

Ionic conductivity is a property where a material is able to conduct electricity through the movement of ions. Oxide ion conductors can be used in solid oxide fuel cells, which can be used to burn fuels more efficiently. High temperature delta-Bi2O3 is the best oxide conductor known with a conductivity of 1 S/cm at 750 °C, but it is only stable from 730 °C to 804 °C. By doping the lanthanides La and Dy, stable structures can be performed with conductivity of 0.01 S/cm at temperatures of 550 °C and 700 °C respectively, outperforming the currently-used yttria stabilised zirconia, which needs a temperature of 800 °C for the same conductivity. The purpose of this experiment is to investigate the structural features on an atomic scale of the materials Bi0.775Ln0.225O1.5 (Ln = La, Dy) to understand why they are good ionic conductors.

Identifier
DOI https://doi.org/10.5286/ISIS.E.84783008
Metadata Access https://icatisis.esc.rl.ac.uk/oaipmh/request?verb=GetRecord&metadataPrefix=oai_datacite&identifier=oai:icatisis.esc.rl.ac.uk:inv/84783008
Provenance
Creator Dr Phil Chater; Professor John Evans; Professor Ivana Evans; Dr Helen Playford; Dr Matthew Chambers; Dr Matthew Tucker
Publisher ISIS Neutron and Muon Source
Publication Year 2020
Rights CC-BY Attribution 4.0 International; https://creativecommons.org/licenses/by/4.0/
OpenAccess true
Contact isisdata(at)stfc.ac.uk
Representation
Resource Type Dataset
Discipline Chemistry; Natural Sciences
Temporal Coverage Begin 2017-03-21T08:00:00Z
Temporal Coverage End 2017-03-23T08:00:00Z