The effect of redox on the substitution mechanism of Ti in meteoritic hibonite

DOI

We request 3 days of beam-time on HRPD to identify the substitution mechanism of Ti3+ and Ti4+ in synthetic hibonites [CaAl12O19]. The experiment forms part of a larger programme in which we are using the Ti3+/Ti4+ ratio as a redox sensor to monitor the evolution of the oxygen fugacity conditions in the early solar system. This work is dependent upon analysis of XAS data from a set of synthetic Ti substituted hibonites that have been prepared under known oxygen fugacity conditions. To perform the XAS analyses successfully we require good structural characterisation of these standards, and we believe that neutron diffraction is the most suitable method available.

Identifier
DOI https://doi.org/10.5286/ISIS.E.24077066
Metadata Access https://icatisis.esc.rl.ac.uk/oaipmh/request?verb=GetRecord&metadataPrefix=oai_datacite&identifier=oai:icatisis.esc.rl.ac.uk:inv/24077066
Provenance
Creator Dr Paul Schofield; Dr Kevin Knight
Publisher ISIS Neutron and Muon Source
Publication Year 2012
Rights CC-BY Attribution 4.0 International; https://creativecommons.org/licenses/by/4.0/
OpenAccess true
Contact isisdata(at)stfc.ac.uk
Representation
Resource Type Dataset
Discipline Photon- and Neutron Geosciences
Temporal Coverage Begin 2009-09-22T07:56:07Z
Temporal Coverage End 2009-09-25T08:38:29Z