Photo-catalytic oxidation of phenol over porous TiO2: A Modulation excitation study

DOI

Solar energy is an abundant renewable source to tackle energy and environmental concerns. For example, solar energy can be converted into electricity, can be used to produce fuels from water and/or CO2 and can be utilised to purify polluted air and water from industrial wastes. These photo-catalytic processes involve a catalyst which plays a crucial role in the efficiency of a process. We study photocatalytic oxidation of organic pollutants, such as phenol, from waste water using a porous TiO2 catalyst. This photo-catalytic process however has low efficiency and produces unwanted by-products which are equally, if not more, harmful than the parent pollutant itself. Therefore, using total neutron scattering, we aim to better understand the local environment of liquids (structure and orientation) within catalyst pores and thereby the reaction mechanism to mitigate unwanted by-products.

Identifier
DOI https://doi.org/10.5286/ISIS.E.RB1910209-1
Metadata Access https://icatisis.esc.rl.ac.uk/oaipmh/request?verb=GetRecord&metadataPrefix=oai_datacite&identifier=oai:icatisis.esc.rl.ac.uk:inv/109730153
Provenance
Creator Dr Santhosh Matam; Professor Chris Hardacre; Dr Tristan Youngs; Dr Sofia Diaz-Moreno; Dr Daniel Bowron; Dr Adam Greer; Mr Armando Ibraliu; Dr Shaojun Xu
Publisher ISIS Neutron and Muon Source
Publication Year 2023
Rights CC-BY Attribution 4.0 International; https://creativecommons.org/licenses/by/4.0/
OpenAccess true
Contact isisdata(at)stfc.ac.uk
Representation
Resource Type Dataset
Discipline Chemistry; Natural Sciences
Temporal Coverage Begin 2020-03-11T11:37:33Z
Temporal Coverage End 2020-03-18T09:58:15Z