Local structures and dynamics of new functional oxides

DOI

The melilite family are new xoide ion conductors with high mobility at low temperatures. Average structures suggest that the ability of the structure to accomodate high levels of interstitials and allow these defects to move with high mobility is due to the presence of tetrahedral centres which are not completely condensed to form the oxide framework. This structural feature would allow relaxation when the defect binds to this centre, and may also, by analogy with the negative thermal expansion materials, produce dynamical features associated with rigid unit modes that enable defect motion. The collection of variable temperature total scattering data will allow the static structure around the defect and the framework dynamics to be investigated using RMC analysis.Lead-free relaxor ferroelectrics are important materials. The local structure of a new example will be analysed.

Identifier
DOI https://doi.org/10.5286/ISIS.E.24079390
Metadata Access https://icatisis.esc.rl.ac.uk/oaipmh/request?verb=GetRecord&metadataPrefix=oai_datacite&identifier=oai:icatisis.esc.rl.ac.uk:inv/24079390
Provenance
Creator Professor Martin Dove; Dr Matthew Rosseinsky; Dr John Claridge; Dr Matthew Tucker; Mr Robert Szczecinski; Dr Katherine Thompson; Dr Sam Chong
Publisher ISIS Neutron and Muon Source
Publication Year 2013
Rights CC-BY Attribution 4.0 International; https://creativecommons.org/licenses/by/4.0/
OpenAccess true
Contact isisdata(at)stfc.ac.uk
Representation
Resource Type Dataset
Discipline Photon- and Neutron Geosciences
Temporal Coverage Begin 2010-07-06T09:49:41Z
Temporal Coverage End 2010-07-15T08:58:18Z