Investigating methods to create cavities within templated electrodeposited polymers using off-specular reflectivity

DOI

Nanoporous membranes are widely used in (bio)sensors, chromatography, charge storage devices, filtration and catalysis. With increasing efforts to develop microfabricated sytem- or lab-on-a-chip devices that perform a wide range of functions, there is a need to devise in situ methods to incorporate elements such as membranes. A suitable in-situ fabrication method is electropolymerisation of monomer units around templates that are subsequently eluted. However, whilst this strategy can be depicted in a cartoon, direct morphological characterisation of any subsurface cavities is notoriously difficult. Often desirable pores are ~20-200 nm and thus on the length scale accessible with offspecular reflectivity on OFFSPEC. Therefore here we seek to use this technique to probe the number density and size of cavities generated by an elution strategy, thereby adding quantification to the cartoon.

Identifier
DOI https://doi.org/10.5286/ISIS.E.53843099
Metadata Access https://icatisis.esc.rl.ac.uk/oaipmh/request?verb=GetRecord&metadataPrefix=oai_datacite&identifier=oai:icatisis.esc.rl.ac.uk:inv/53843099
Provenance
Creator Dr Andrew Glidle; Dr Huabing Yin; Professor Jon Cooper; Professor Karl Ryder; Professor Robert Hillman; Dr Robert Dalgliesh
Publisher ISIS Neutron and Muon Source
Publication Year 2017
Rights CC-BY Attribution 4.0 International; https://creativecommons.org/licenses/by/4.0/
OpenAccess true
Contact isisdata(at)stfc.ac.uk
Representation
Resource Type Dataset
Discipline Photon- and Neutron Geosciences
Temporal Coverage Begin 2014-06-11T23:00:00Z
Temporal Coverage End 2014-06-16T08:06:45Z