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Understanding the spin-Peierls Transition in KTCNQ and derivatives
Motivated by work showing that magnetic coupling between TCNQ anions in potassium TCNQ (KTCNQ) can be changed simply by changing the aromatic substituents, we seek to qunatify... -
Probing the spin dynamics in the pseudo-quaternary Y1-xErxNi2B2C compounds
Our uSR measurements on superconducting Y1-xErxNi2B2C shows a slowing of the Er spin dynamics upon cooling to 2.5 K, but the depolarisation rate does not critically diverge and... -
The search and optimisation of Delta0 resonances in TIPS-Pentacene in solution
To the best of our knowledge, there is no previous work on using muons to measure photo-excited states in organic semiconductors or related materials. Our photo-excitation ideas... -
characterisation of muonium in functionalized acenes
We wish to measure the high field ALCs of a series of related functionalised acenes, to understand the role of the ligands on the electron spin relaxation, which is of... -
Spin Rotation Experiments at a Pulsed Muon Source using Broadband RF Pulses
In this proposal we wish to explore how the RF-MuSR technique might be developed for measurements akin to FT-NMR. Our work will focus on the broadband excitation of paramagnetic... -
RF-muSR in the gas phase: the muoniated ethyl radical
Radio-frequency muon spin resonance is an exceptional technique for studying free radicals, but it has not been applied to study radicals in the gas phase. In a previous... -
Artificial [FeFe]-Hydrogenases and Muon Spectroscopy
Preliminary measurements of [FeFe]-hydrogenase model complexes were made in a previous experiment using EMU (RB 1010177). The results were interpreted in combination with DFT... -
Muon Spin Relaxation and ALC Resonance in Magnetic and non-Magnetic Oxalate S...
Repolarisation and level crossing resonance will be studied for several different oxalate compounds where muon radical states are known to be formed. Such compounds form a... -
Muon level-crossing resonances as a probe for studying antiferromagnets at pu...
We propose a set of measurements using the HiFi spectrometer in which muon level-crossing resonances are used to probe the internal field inside antiferromagnets in which the... -
Hunting for the low-temperature, low-field magnetization plateau in Tb2Ti2O7
Tb2Ti2O7 is a pyrochlore antiferromagnet that has previously been viewed as a spin liquid. This description fails to describe key features of its physics and more recently the... -
Using muons to investigate the excitation spectrum in low-dimensional molecul...
We propose to use longitudinal field muon-spin relaxation to investigate the excitation spectrum of the most successful realizations of one- and two-dimensional antiferromagnets... -
Unconventional superconductivity in quasi-1D K_2Cr_3As_3 (QLCR)
Metallic systems with one-dimensional chain-like atomic structure can support unusual mechanisms for electron pairing leading to superconductivity. K_2Cr_3As_3 is one of a... -
Muon level-crossing resonances as a probe for studying antiferromagnets at pu...
We propose a set of measurements using the HiFi spectrometer in which muon level-crossing resonances are used to probe the internal field inside antiferromagnets in which the... -
Study of electron spin relaxation in the anthradithiophene series, substitute...
The emerging field of organic spintronics is especially promising for new technologies, owing to the long spin coherence times, large flexibility and low production costs of the... -
Muonium and Flourine Entangled States In An Organic Based Spin Peierls System
Potassium TCNQ is an stoichiometric organic based salt that undergoes a spin Peierls (SP) transition at approximately 390 K. Much research has been conducted on this system in... -
Development of Radio Frequency µSR as a Method for Determining Hyperfine Coup...
Radio Frequency µSR provides a direct method for accurately determining muon hyperfine coupling constants, Aµ, for muoniated radical species. The method complements the well... -
Study of the dependence of electron spin relaxation on molecule length in acenes
We wish to measure the ALCs of a series of polyacene molecules made of a different number of rings. We would like to identify the dependence of the electron spin relaxation rate... -
Utilising Quadrupolar Level Crossing Resonance to Gain Important Information ...
There is much debate about muon stopping sites within materials and in many cases knowing where the muon stops is crucial to understanding the physical properties of different... -
End-Game: Cornering Solvent Effects on H-Addition in Green Tea Anti-Oxidants
Our ongoing project to characterise radical scavenging by the green tea anti-oxidant EGCG and its D-ring analogue, (3,4,5-(OH)3-Bz) is near-complete. ALC-MuSR experiments on the... -
Multiferroicity in metal-formate perovskites
Recent work has revealed that metal-organic frameworks (MOFs) can also exhibit this multiferroicity. These materials are particularly interesting since their structures are...
