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Understanding the spin-Peierls Transition in KTCNQ and derivatives
Motivated by work showing that magnetic coupling between TCNQ anions in potassium TCNQ (KTCNQ) can be changed simply by changing the aromatic substituents, we seek to qunatify... -
Frustration, quantum spin ices and quantum diffusion
This proposal aims to characterise the spin dynamics of three Pr-based pyrochlores that may be realisations of quantum spin ice materials. The lower moment and larger wave... -
DYNAMICS OF SURFACTANTS IN LUBRICATING OILS
In a recent series of successful experiments at PSI and ISIS we were able to demonstrate the possibility of measuring the rate of transfer of a small molecule (allyl alcohol)... -
Spin relaxation of short-lived spin-labelled radicals in solution
The spin relaxation rates of free radicals in solution can provide valuable information about the dynamics of molecular tumbling in solution, and solvent-radical interactions.... -
Understanding Li-Diffusion and Resultant Magnetism Within Li Intercalated int...
This study involves attempting to understand the Li atom diffusion within Li-intercalated hexagonal boron nitride. Muons present a significant advantage as they are sensitive to... -
Spin Rotation Experiments at a Pulsed Muon Source using Broadband RF Pulses
In this proposal we wish to explore how the RF-MuSR technique might be developed for measurements akin to FT-NMR. Our work will focus on the broadband excitation of paramagnetic... -
Muon Spin Relaxation studies of Ni2TCNQ, Ni(TCNQ)2 and related materials
Amorphous molecular magnetic materials Ni2(OA) (OA:organic acceptor) were reported to exhibit ferromagnetism with Curie temperatures >400K. This work is controversial as it... -
muSR in the presence of significant spin-orbit coupling
The great majority of known muonium defect centres and muonium substituted organic radicals have essentially spin-only magnetism, with few exhibiting any noticeable departure... -
ALC measurments on deuterated TCNQ
This dataset has no description
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Muonium in alpha-boron
Previous muon experiments have identified a muonium state in the commonly occuring, but complex, beta rhombohedral form of elemental boron. To complement recent theoretical work... -
Investigation of carrier transport in the organic semiconductor 8-hydroxy-qui...
Using the Emu spectrometer at ISIS we have recently studied charge carrier transport in the technologically important molecule 8-hydroxy-quinoline aluminium, by probing the... -
Understanding Spin Density Variations in Fluorinated TCNQ Adducts
There is a large emphisis on fucntialising materials to create magnetic and electrical materials. Tetracyanoquinodimethane is a famous material discovered in the 1960 and ws... -
The XY pyrochlore AFM:spin dynamics upon rare-earth dilution in Er2Ti2O7 (CON...
Er2Ti2O7 constitutes an experimental realization of the <111> easy-plane pyrochlore AFM and orders at 1.1 K into the theoretically predicted spin structure. However, the... -
Multiferroicity in metal-formate perovskites
Recent work has revealed that metal-organic frameworks (MOFs) can also exhibit this multiferroicity. These materials are particularly interesting since their structures are... -
End-Game: Cornering Solvent Effects on H-Addition in Green Tea Anti-Oxidants
Our ongoing project to characterise radical scavenging by the green tea anti-oxidant EGCG and its D-ring analogue, (3,4,5-(OH)3-Bz) is near-complete. ALC-MuSR experiments on the... -
Utilising Quadrupolar Level Crossing Resonance to Gain Important Information ...
There is much debate about muon stopping sites within materials and in many cases knowing where the muon stops is crucial to understanding the physical properties of different... -
Study of the dependence of electron spin relaxation on molecule length in acenes
We wish to measure the ALCs of a series of polyacene molecules made of a different number of rings. We would like to identify the dependence of the electron spin relaxation rate... -
Development of Radio Frequency µSR as a Method for Determining Hyperfine Coup...
Radio Frequency µSR provides a direct method for accurately determining muon hyperfine coupling constants, Aµ, for muoniated radical species. The method complements the well... -
Muonium and Flourine Entangled States In An Organic Based Spin Peierls System
Potassium TCNQ is an stoichiometric organic based salt that undergoes a spin Peierls (SP) transition at approximately 390 K. Much research has been conducted on this system in... -
Study of electron spin relaxation in the anthradithiophene series, substitute...
The emerging field of organic spintronics is especially promising for new technologies, owing to the long spin coherence times, large flexibility and low production costs of the...
