INS study of the effect of particle size on the formation of beta-palladium hydride

DOI

Finely divided, supported palladium particles are used as catalysts in many technical processes. However, there is still considerable potential to improve catalyst performance and selectivity. Important parameters that can be fine-tuned are the size, distribution and shape of the primary particles as appropriate for the particular application or process. We propose to measure nano-scale palladium particles supported on special grades of activated carbon. The samples are three Pd(5 wt%) on activated carbon catalysts of different average primary particle size (2, 3, 5 nm). Comparison between the samples should reveal: different site occupation (100)/(111) by hydrogen and changes of long range phase coherence in the 2-5 nm particle regime and, therefore, incomplete formation of the beta-phase PdH. The tenfold sensitivity advantage of MAPS over TOSCA is essential to these measurements.

Identifier
DOI https://doi.org/10.5286/ISIS.E.24079556
Metadata Access https://icatisis.esc.rl.ac.uk/oaipmh/request?verb=GetRecord&metadataPrefix=oai_datacite&identifier=oai:icatisis.esc.rl.ac.uk:inv/24079556
Provenance
Creator Professor Stewart Parker; Dr Peter Albers
Publisher ISIS Neutron and Muon Source
Publication Year 2013
Rights CC-BY Attribution 4.0 International; https://creativecommons.org/licenses/by/4.0/
OpenAccess true
Contact isisdata(at)stfc.ac.uk
Representation
Resource Type Dataset
Discipline Photon- and Neutron Geosciences
Temporal Coverage Begin 2010-07-23T18:11:51Z
Temporal Coverage End 2010-08-01T12:04:35Z