Generalized DeepONets for Viscosity Prediction Using Learned Entropy Scaling References

DOI

Data-driven approaches used to predict thermophysical properties benefit from physical constraints because the extrapolation behavior can be improved and the amount of training data be reduced. In the present work, the well-established entropy scaling approach is incorporated into a neural network architecture to predict the shear viscosity of a diverse set of pure fluids over a large temperature and pressure range. Instead of imposing a particular form of the reference entropy and reference shear viscosity, these properties are learned. The resulting architecture can be interpreted as two linked DeepONets with generalization capabilities.

Identifier
DOI https://doi.org/10.18419/DARUS-5256
Related Identifier IsSupplementTo https://doi.org/10.26434/chemrxiv-2025-jrjj9
Metadata Access https://darus.uni-stuttgart.de/oai?verb=GetRecord&metadataPrefix=oai_datacite&identifier=doi:10.18419/DARUS-5256
Provenance
Creator Fleck, Maximilian ORCID logo; Spera, Marcelle ORCID logo; Darouich, Samir ORCID logo; Klenk, Timo; Hansen, Niels ORCID logo
Publisher DaRUS
Contributor Hansen, Niels
Publication Year 2025
Funding Reference DFG EXC 2075 - 390740016
Rights CC BY 4.0; info:eu-repo/semantics/openAccess; http://creativecommons.org/licenses/by/4.0
OpenAccess true
Contact Hansen, Niels (University of Stuttgart)
Representation
Resource Type Dataset
Format application/zip
Size 2051492329
Version 1.0
Discipline Chemistry; Construction Engineering and Architecture; Engineering; Engineering Sciences; Natural Sciences