Discriminating adsorption sites in the coordinatively unstaurated 3d metal ion MOF CPO-27-Fe

DOI

Using chemically different substances as co-adsorbates allows one to block certain types of adsorption sites in a given porous material or even on a surface. This can be very useful for distinguishing and identifying various different adsorption sites in an heterogenous adsorbent. It has also the potential of helping in better and more reliable interpretation of inelastic neutron scattering spectra of adsorbed dihydrogen for instance. Particularly useful the technique can be where different set of sites with very similar adsortpion heats are present or different types dihydrogen complexes on a certen complex forming centre may be present. In the case of the CPO-27-Fe, preadsorption of O2 can be used to poison the "metal" sites located just above the Fe(II) ion by forming a stable Fe(II)-O2 oxocomplex, then dose H2, and re-measure an INS spectrum free of Fe(II) sites contribution.

Identifier
DOI https://doi.org/10.5286/ISIS.E.24088869
Metadata Access https://icatisis.esc.rl.ac.uk/oaipmh/request?verb=GetRecord&metadataPrefix=oai_datacite&identifier=oai:icatisis.esc.rl.ac.uk:inv/24088869
Provenance
Creator Professor Alberto Albinati; Dr Peter Georgiev; Professor Pascal Dietzel
Publisher ISIS Neutron and Muon Source
Publication Year 2015
Rights CC-BY Attribution 4.0 International; https://creativecommons.org/licenses/by/4.0/
OpenAccess true
Contact isisdata(at)stfc.ac.uk
Representation
Resource Type Dataset
Discipline Photon- and Neutron Geosciences
Temporal Coverage Begin 2012-05-29T07:52:42Z
Temporal Coverage End 2012-06-04T06:53:26Z