Ordering in La/W Double Substituted Bismuth Oxide Based Fluorites

DOI

Materials that show fast oxide ion conduction have potential applications as electrolytes in devices such as solid oxide fuel cells (SOFCs), gas sensors and gas separation membranes. While bismuth oxide shows the highest oxide ion conductivity of any material it can only be stabilised at lower temperatures through partial substitution of bismuth by other cations. A total scattering study of W and La substituted bismuth oxide based electrolytes is proposed, with a view to examining details of local coordination and vacancy ordering. Fluorite based phases will be examined in two solid solution systems. Both systems show a highly conducting fully disordered delta-Bi2O3 type phase at elevated temperature, which can be stabilised to room temperature depending on composition. The results from the proposed study will be used to shed light on the conduction mechanisms in these systems.

Identifier
DOI https://doi.org/10.5286/ISIS.E.83551235
Metadata Access https://icatisis.esc.rl.ac.uk/oaipmh/request?verb=GetRecord&metadataPrefix=oai_datacite&identifier=oai:icatisis.esc.rl.ac.uk:inv/83551235
Provenance
Creator Dr Marcin Malys; Mr Ali Shehu; Dr Ron Smith; Dr Anna Borowska; Dr Stefan Norberg; Dr Steve Hull; Dr Isaac Abrahams; Professor Franciszek Krok
Publisher ISIS Neutron and Muon Source
Publication Year 2019
Rights CC-BY Attribution 4.0 International; https://creativecommons.org/licenses/by/4.0/
OpenAccess true
Contact isisdata(at)stfc.ac.uk
Representation
Resource Type Dataset
Discipline Photon- and Neutron Geosciences
Temporal Coverage Begin 2016-11-17T08:00:00Z
Temporal Coverage End 2016-11-20T08:00:00Z