Magnetic order in the triangular quantum magnet AgNiO2

DOI

This proposal is part of our research programme on spin and orbital order in frustrated systems. AgNiO2 has a layered crystal structure with Jahn-Teller active Ni3+ ions forming an antiferromagnetic triangular lattice in the basal plane. Both spin and orbital order are frustrated in this geometry and unusual ground states may occur. There are two structural polytypes which differ in the stacking of NiO2 layers. We have observed a complex supercell structure in the hexagonal polytype with a novel magnetic ground state with ordered spins arranged in alternating stripes surrounded by unordered sites. Surprisingly the orbital degeneracy is lifted not by Jahn-Teller distortions as in other triangular spin-orbital systems but by charge order. Here we wish to explore the magnetic order in the rhombohedral polytype, where interlayer interactions are different and a new ground state is expected.

Identifier
DOI https://doi.org/10.5286/ISIS.E.24003335
Metadata Access https://icatisis.esc.rl.ac.uk/oaipmh/request?verb=GetRecord&metadataPrefix=oai_datacite&identifier=oai:icatisis.esc.rl.ac.uk:inv/24003335
Provenance
Creator Professor Radu Coldea; Dr Elisa Wheeler; Dr Ewa Wawrzynska
Publisher ISIS Neutron and Muon Source
Publication Year 2011
Rights CC-BY Attribution 4.0 International; https://creativecommons.org/licenses/by/4.0/
OpenAccess true
Contact isisdata(at)stfc.ac.uk
Representation
Resource Type Dataset
Discipline Photon- and Neutron Geosciences
Temporal Coverage Begin 2008-02-08T00:52:29Z
Temporal Coverage End 2008-02-09T08:52:46Z