Unveiling the boundaries of mesodomains formation in the monophasic region of ternary phase diagrams

DOI

Liquid mixtures of simple solvents can form nanosized clusters, even relatively far away from their critical point. We propose to revisit the monophasic region of these seemingly simple mixtures, as the mesoscale inhomogeneities they exhibit can explain unusual chemical (re)activity, solubilisation properties etc. We focus on the case of ternary mixtures where two largely immiscible fluids are homogenised with the addition of a solvotrope. We will determine the location of two important pseudo-phase boundaries that we identify as the Lifshitz line and the Widom line, in two similar ternary mixtures: water/ethanol/1-octanol and water/ethanol/2-ethyl-1-hexanol. The later is an isomer of 1-octanol, with a greater propensity for self-aggregation in the form of rings rather than chains, making it far more difficult to pack. We will map the phase diagrams by in situ auto-dilution, and will complete our study with temperature scans to characterize the critical exponents of these systems.

Identifier
DOI https://doi.org/10.15151/ESRF-ES-894942586
Metadata Access https://icatplus.esrf.fr/oaipmh/request?verb=GetRecord&metadataPrefix=oai_datacite&identifier=oai:icatplus.esrf.fr:inv/894942586
Provenance
Creator Marie PLAZANET; Ingo HOFFMANN; Peter BOESECKE; Christiane ALBA-SIMIONESCO; Firoz MALAYIL KALATHIL; Sylvain PREVOST
Publisher ESRF (European Synchrotron Radiation Facility)
Publication Year 2025
Rights CC-BY-4.0; https://creativecommons.org/licenses/by/4.0
OpenAccess true
Representation
Resource Type Data from large facility measurement; Collection
Discipline Particles, Nuclei and Fields