Disorder-resilient transition of Helical to Conical ground states in M<sub>1/3</sub>NbS<sub>2</sub>, M=Cr,Mn

DOI

The discovery of chiral helical magnetism (CHM) in Cr<sub>1/3</sub>NbS<sub>2</sub> and the stabilization of a chiral soliton lattice (CSL) has attracted considerable interest in view of their potential technological applications. However, there is an ongoing debate regarding whether the sister compound, Mn<sub>1/3</sub>NbS<sub>2</sub>, which shares the same crystal structure, exhibits similar nontrivial properties, which rely on the stabilization of the lack of inversion symmetry at the magnetic ion. In this study, we conduct a comprehensive investigation of the magnetically ordered states of both compounds, using <sup>53</sup>Cr, <sup>55</sup>Mn and <sup>93</sup>Nb nuclear magnetic resonance. Our results, supported by density functional calculations, detect in a high quality single crystal of Cr<sub>1/3</sub>NbS<sub>2</sub> all the signatures of the monoaxial CHM in a magnetic field, identifying it as a textbook NMR case. The detailed understanding of this prototypic behavior provides a reference for Mn<sub>1/3</sub>NbS<sub>2</sub>. Despite the much larger density of specific defects in this second single crystal, we confirm the presence of a CHM phase in the Mn compound, characterized by a very large critical field for the forced ferromagnetic phase (~ 10 T for H || c).

Identifier
DOI https://doi.org/10.24435/materialscloud:6v-9v
Related Identifier https://doi.org/10.48550/arXiv.2410.01631
Related Identifier http://arxiv.org/abs/2410.01631
Related Identifier https://archive.materialscloud.org/communities/mcarchive
Related Identifier https://doi.org/10.24435/materialscloud:et-9z
Metadata Access https://archive.materialscloud.org/oai2d?verb=GetRecord&metadataPrefix=oai_dc&identifier=oai:materialscloud.org:2290
Provenance
Creator Sahoo, Manaswini; Bonfà, Pietro; Hall, Amelia Elisabeth; Mayoh, Daniel A.; Corredor, Laura Teresa; Wolter, Anja U. B.; Büchner, Bernd; Balakrishnan, Geetha; De Renzi, Roberto; Allodi, Giuseppe
Publisher Materials Cloud
Contributor Sahoo, Manaswini; Bonfà, Pietro
Publication Year 2024
Rights info:eu-repo/semantics/openAccess; Creative Commons Attribution 4.0 International; https://creativecommons.org/licenses/by/4.0/legalcode
OpenAccess true
Contact archive(at)materialscloud.org
Representation
Language English
Resource Type info:eu-repo/semantics/other
Format application/gzip; text/markdown
Discipline Materials Science and Engineering