Capturing Structural Evolution and Reaction Intermediates in (Mn-Nb)O2-F During the Electrochemical OER with Time-Resolved XAS

DOI

Proton Exchange Membrane Water Electrolysis (PEMWE) is crucial for hydrogen production but relies on scarce platinum group metals (PGMs) like platinum (Pt) and iridium oxide (IrO₂), limiting scalability. A key challenge is the sluggish oxygen evolution reaction (OER) and poor anode stability in acidic conditions, affecting efficiency.[1,2] This work aims to gain a thorough mechanistic understanding of a stable and active PGM-free OER catalyst based on manganese (Mn)-based material doped with niobium (Nb) and fluorine (F). Electrochemical operando XAS will probe catalyst’s structural and electronic properties, revealing how Nb and F enhance stability and activity in PEMWE.

Identifier
DOI https://doi.org/10.15151/ESRF-ES-2220632850
Metadata Access https://icatplus.esrf.fr/oaipmh/request?verb=GetRecord&metadataPrefix=oai_datacite&identifier=oai:icatplus.esrf.fr:inv/2220632850
Provenance
Creator Anna SCOTT (ORCID: 0009-0000-5803-691X); Vimanshu CHANDA; Davide SALUSSO ORCID logo; Olaf RUEDIGER ORCID logo; Sergio JANNUZZI ORCID logo
Publisher ESRF (European Synchrotron Radiation Facility)
Publication Year 2028
Rights CC-BY-4.0; https://creativecommons.org/licenses/by/4.0
OpenAccess true
Representation
Resource Type Data from large facility measurement; Collection
Discipline Particles, Nuclei and Fields