An automatic robotic Lift (RoLi) was used to measure vertical profiles (8.3 - 318.3 m) of basic meteorological parameters and atmospheric aerosol characteristics at the 325 m tall ATTO Tower, located at the Amazon Tall Tower Observatory in Brazil (ATTO, -59.005626 E, -2.145898 N). This dataset includes exemplary measurements collected on January 8, 2023, and between April 24 and April 28, 2024. The technical information about RoLi can be found at 'Automated atmospheric profiling with the Robotic Lift (RoLi) at the Amazon Tall Tower Observatory', Brill et al., 2025 (https://doi.org/10.5194/egusphere-2025-295). File format: Files are ASCII files containing tab-separated tables, cf "https://doi.org/10.17617/3.10" for details.