In-depth understanding coking in dry reforming of methane on Ni-Co bimetallic catalysts

DOI

Ni-Co bimetallic catalysts significantly outperform to individual monmetallic catalysts for dry reforming of methane using CO2, in particular in the resistance to carbon deposition (coking) and thus prolonged catalyst lifetime. However the function of individual metals remains uncertain and the mechanistic scheme of coking necessitate to uncover. As proved in literatures, Inelastic neutron scattering (INS) technique provides powerful tools to analyse the carbonaceous species formed in the dry reforming, pecularly useful to determine the participation of hydrogen which is impossible to be clarified by IR or Raman, in the spent catalysts. The support effects can also be explored via such powerful INS technique. We will conduct INS experiements for 32 Ni-Co alloy catalysts supported on Al2O3, TiO2, CeO2 and Spinel (8 samples on each support) to clarify effects of alloy and supports.

Identifier
DOI https://doi.org/10.5286/ISIS.E.49920370
Metadata Access https://icatisis.esc.rl.ac.uk/oaipmh/request?verb=GetRecord&metadataPrefix=oai_datacite&identifier=oai:icatisis.esc.rl.ac.uk:inv/49920370
Provenance
Creator Dr Zheng Jiang; Dr Lina Chi; Mr Xin Liao; Professor Stewart Parker
Publisher ISIS Neutron and Muon Source
Publication Year 2017
Rights CC-BY Attribution 4.0 International; https://creativecommons.org/licenses/by/4.0/
OpenAccess true
Contact isisdata(at)stfc.ac.uk
Representation
Resource Type Dataset
Discipline Chemistry; Construction Engineering and Architecture; Engineering; Engineering Sciences; Natural Sciences; Physics
Temporal Coverage Begin 2014-08-03T23:00:00Z
Temporal Coverage End 2014-08-06T23:00:00Z