Kinetic study of phase transformations in the deuterated Pd/Ag alloy

DOI

Hydrogen selective palladium membranes are important for technological processes of H separation and purification, but they become brittle because of repeated alpha - beta phase transformations. Pd is usually alloyed with Ag to avoid this membrane embrittlement, assuming a single-phase behaviour during hydrogenation. However, in the previous experiment 5-25-247 on D2B, in-situ measurements on Pd0.77Ag0.23D x at variable T and p(D2) revealed a transformation between two FCC phases with different lattice constants and deuterium contents, depending on time and high-pressure pre-treatments. The D-poorer phase seems to be metastable and to transform progressively into the D-richer one. An experiment is thus proposed on the high-resolution high-intensity D20 diffractometer, with the aim of studying the kinetics of this process. Two days are requested, to collect series of 20 consecutive patterns at 80 and 160 °C, and pressures in the 1 to 12 bar range, including the study of baric history effects.

Identifier
DOI https://doi.org/10.5291/ILL-DATA.5-25-260
Metadata Access https://data.ill.fr/openaire/oai?verb=GetRecord&metadataPrefix=oai_datacite&identifier=10.5291/ILL-DATA.5-25-260
Provenance
Creator Filabozzi, Alessandra; Santucci, Alessia; Pietropaolo, Antonino; Catti, Michele; Rosa, Oscar Ramon Fabelo; Tosti, Silvano
Publisher Institut Laue-Langevin
Publication Year 2018
Rights OpenAccess; info:eu-repo/semantics/openAccess
OpenAccess true
Representation
Resource Type Dataset
Size 264 MB
Version 1
Discipline Particles, Nuclei and Fields