Unraveling density profiles leading to antifouling surfaces

DOI

We propose to study the density profiles of the non-fouling poly[N-(2-hydroxypropyl) methacrylamide] (poly(HPMA)) and antifouling poly[oligo(ethylene glycol)methyl ether methacrylate] (poly(MeOEGMA)) brushes at the solid-liquid interface by neutron reflectivity. The solvent-swollen brushes will be measured before and after contact with fibrinogen solution and whole blood plasma, at 25 and 37ºC at different contrast. Studies the brush profiles at different temperature will determine the importance of entropy on the resistance to fouling, while assessing the profiles after protein adsorption will aid at assessing whether fouling leads to changes in the conformation of the brush with a concomitant entropic penalty. The differences between the molecular conformations of the chains between poly(HPMA) and poly(MeOEGMA) brushes will help us to identify the key parameters rendering a surface non-fouling. Thus the obtained results will enable us to design synthetic protocols for surface modifications with predictable and tailor-made properties.

Identifier
DOI https://doi.org/10.5291/ILL-DATA.9-12-386
Metadata Access https://data.ill.fr/openaire/oai?verb=GetRecord&metadataPrefix=oai_datacite&identifier=10.5291/ILL-DATA.9-12-386
Provenance
Creator De Los Santos Pereira, Andres; Emmenegger, Cesar Rodriguez; Trapp, Marcus; Ballauff, Matthias; Gutfreund, Philipp; Steitz, Roland
Publisher Institut Laue-Langevin
Publication Year 2015
Rights OpenAccess; info:eu-repo/semantics/openAccess
OpenAccess true
Representation
Resource Type Dataset
Size 2 GB
Version 1
Discipline Particles, Nuclei and Fields