XMCD study of the first-order magnetization process in U3Cu4Ge4

DOI

U3Cu4Ge4 is a ferromagnet with the magnetic moments aligned along the [100] axis of the orthorhombic crystal structure. When magnetic field is applied along the hard [010] direction, U3Cu4Ge4 displays a firstorder phase transition in the magnetization at H = 25 T. This phase transition occurs due to the existence of two inequivalent minima in the magnetic-anisotropy energy of the material and reflects a strong response of the 5f electrons. Our magnetization and ultrasound data strongly suggest a Fermi-surface reconstruction and lattice deformation at H. Here, we propose to perform orbital-selective magnetometry through x-ray magnetic circular dichroism at the U L3 edge to determine the microscopic nature of the field-induced transition. Our goal is to analyze dipolar and quadrupolar contributions in the U L3 edge XMCD in order to resolve the degree of localization of the 5f electrons in U3Cu4Ge4.

Identifier
DOI https://doi.org/10.15151/ESRF-ES-1022934262
Metadata Access https://icatplus.esrf.fr/oaipmh/request?verb=GetRecord&metadataPrefix=oai_datacite&identifier=oai:icatplus.esrf.fr:inv/1022934262
Provenance
Creator Yimin MIJITI ORCID logo; Raffaella TORCHIO; Shingo YAMAMOTO ORCID logo; Fabienne DUC ORCID logo; Cornelius STROHM; Denis GORBUNOV
Publisher ESRF (European Synchrotron Radiation Facility)
Publication Year 2026
Rights CC-BY-4.0; https://creativecommons.org/licenses/by/4.0
OpenAccess true
Representation
Resource Type Data from large facility measurement; Collection
Discipline Particles, Nuclei and Fields