This dataset contains many strongly polarized solar lines belonging to the “second solar spectrum”, i.e. the spectrum near the limb in linear scattering polarization. The observations were done at the Pic du Midi Turret Dome in 2006. The solar spectra were recorded at high spectral resolution (R = 400000) with the spectrograph slit orthogonal to the solar limb, so that µ = cosθ continuously varied from 0.0 to 0.45. The crystal liquid polarimeter delivered the linear polarization rate (Q/I). Strong lines such as CaII 3934 Å, CaI 4227 Å, SrI 4607 Å, SrII 4078 Å, BaII 4554 Å were studied. We measured the Hanle depolarization with the help of models predicting the polarization envelope with no magnetic field and we got values in the range 13-25 Gauss for the unresolved turbulent magnetic field, and we found that it often decreases towards the limb, revealing an altitude gradient. The processed spectra of this dataset are available to the research community.