Light Atom Location in Filled Skutterudites

DOI

Thermoelectric materials offer tremendous potential for the conversion of waste heat energy into useful electrical energy. We are currently engaged on a collaborative project that seeks to develop skutterudites for energy recovery in vehicle exhaust streams. In the course of this work, we have succeeded in introducing lithium filler atoms into a series of isoelectronic mixed-metal skutterudites. This produces significant changes in electrical and thermal transport properties. However, owing to the low X-ray scattering power of lithium we are unable to locate the filler atom by X-ray methods. We wish to exploit the capacity of neutrons to locate lithium in the presence of heavy atoms, to carry out a detailed structural study of a series of isostructural lithium-containing skutterudites.

Identifier
DOI https://doi.org/10.5286/ISIS.E.73944269
Metadata Access https://icatisis.esc.rl.ac.uk/oaipmh/request?verb=GetRecord&metadataPrefix=oai_datacite&identifier=oai:icatisis.esc.rl.ac.uk:inv/73944269
Provenance
Creator Dr Jesus Prado-Gonjal; Professor Anthony Powell; Dr Paz Vaqueiro-Rodriguez; Dr Ron Smith
Publisher ISIS Neutron and Muon Source
Publication Year 2019
Rights CC-BY Attribution 4.0 International; https://creativecommons.org/licenses/by/4.0/
OpenAccess true
Contact isisdata(at)stfc.ac.uk
Representation
Resource Type Dataset
Discipline Chemistry; Natural Sciences
Temporal Coverage Begin 2016-02-29T08:00:00Z
Temporal Coverage End 2016-03-01T08:00:00Z