Vibrational Spectroscopy Studies of Porous Materials for High Capacity Ammonia Storage

DOI

The development of new porous metal-organic frameworks (MOFs) is receiving considerable attention worldwide owing to their potential for gas storage, separation, and purification. We seek to develop highly robust ammonia storage systems for portable applications and request 5 days on TOSCA to study the binding interaction between adsorbed ammonia molecules (NH3) and a robust porous MOF material [NOTT-300(Al)] as a function of NH3 loading. This proposed study will investigate the vibrational properties exhibited by both adsorbed gas substrates and the porous hosts. NOTT-300-Al exhibit high storage capacity for ammonia at ambient conditions (10.2 mmol/g) and more importantly fully reversible uptake, suggesting the presence of specific guest-host interaction. The proposed study aims to reveal the nature of the ammonia uptakes by analysing their vibrational/rotational spectra.

Identifier
DOI https://doi.org/10.5286/ISIS.E.73943917
Metadata Access https://icatisis.esc.rl.ac.uk/oaipmh/request?verb=GetRecord&metadataPrefix=oai_datacite&identifier=oai:icatisis.esc.rl.ac.uk:inv/73943917
Provenance
Creator Professor Sihai Yang; Mr Pete Rought; Dr Svemir Rudic; Mr Harry Godfrey; Professor Martin Schroder; Professor Bill David; Professor Stewart Parker
Publisher ISIS Neutron and Muon Source
Publication Year 2019
Rights CC-BY Attribution 4.0 International; https://creativecommons.org/licenses/by/4.0/
OpenAccess true
Contact isisdata(at)stfc.ac.uk
Representation
Resource Type Dataset
Discipline Chemistry; Natural Sciences
Temporal Coverage Begin 2016-02-17T09:00:00Z
Temporal Coverage End 2016-02-22T09:00:00Z