Spin dynamics and magnetic ordering in the p-orbital molecular solids CsO2 and NaO2

DOI

A magnetic response of the alkali-metal superoxides comes from the p-orbital S = 1/2 spins of anionic O2- molecules. As the O2- molecules are highly reorientable and the corresponding degenerate p orbitals are prone to orbital ordering, these structurally very simple systems exhibit surprisingly complex physics. In CsO2, the p-orbital ordering leading to the formation of spin-1/2 chains below 70 K and a subsequent low-temperature magnetic ordering below 10 K are well established, but the magnetic structure of the ordered phase remains unknown. In NaO2, our NMR results reveal a series of crossovers between different spin-fluctuating regimes below 180 K, but with no signs of magnetic ordering. To address different spin-fluctuating regimes in CsO2 and NaO2 and to unambiguously answer the questions of the existence of the low-temperature magnetic order in NaO2, we are proposing a muSR study.

Identifier
DOI https://doi.org/10.5286/ISIS.E.82355393
Metadata Access https://icatisis.esc.rl.ac.uk/oaipmh/request?verb=GetRecord&metadataPrefix=oai_datacite&identifier=oai:icatisis.esc.rl.ac.uk:inv/82355393
Provenance
Creator Dr Martin Klanjsek; Dr Pabitra Biswas; Dr Martin Jansen; Mr Adler; Dr Denis Arcon; Dr Matjaz Gomilsek; Mr Tilen Knaflic; Dr Andrej Zorko; Dr Peter Adler
Publisher ISIS Neutron and Muon Source
Publication Year 2019
Rights CC-BY Attribution 4.0 International; https://creativecommons.org/licenses/by/4.0/
OpenAccess true
Contact isisdata(at)stfc.ac.uk
Representation
Resource Type Dataset
Discipline Natural Sciences; Physics
Temporal Coverage Begin 2016-10-05T08:30:00Z
Temporal Coverage End 2016-10-08T08:30:00Z