Local Structure within Fluorite-Pyrochlore Solid Solutions

DOI

This proposal requests 6 days beamtime on the Polaris diffractometer to study the nature of the local structure within two systems which have been reported to show a solid solution between pyrochlore and fluorite structure types. The first, Y2(Zr1-yTiy)2O7, shows a gradual transiton from a cation ordered to cation disordered arrangement as Zr content increases, forming an anion-deficient fluorite arrangement. In the second, Ce2Zr2O7+y, the replacement of Ce3+ with Ce4+ leads to a gradual increase in oxygen content, though the pyrochlore cation ordering remains even at the fluorite stoichiometry (Ce2Zr2O8). However, previous work on both these systems has focussed on the averaged structure and, to provide a detailed insight into the nature of the local co-ordinations around the various cation species, we shall perform reverse Monte Carlo modelling of the total scattering data

Identifier
DOI https://doi.org/10.5286/ISIS.E.24079444
Metadata Access https://icatisis.esc.rl.ac.uk/oaipmh/request?verb=GetRecord&metadataPrefix=oai_datacite&identifier=oai:icatisis.esc.rl.ac.uk:inv/24079444
Provenance
Creator Dr Steve Hull; Professor Sten Eriksson; Dr Istaq Ahmed; Dr Stefan Norberg
Publisher ISIS Neutron and Muon Source
Publication Year 2013
Rights CC-BY Attribution 4.0 International; https://creativecommons.org/licenses/by/4.0/
OpenAccess true
Contact isisdata(at)stfc.ac.uk
Representation
Resource Type Dataset
Discipline Photon- and Neutron Geosciences
Temporal Coverage Begin 2010-07-21T14:02:55Z
Temporal Coverage End 2010-07-26T05:26:05Z