Comparative study on Li diffusion in Li-Ti-oxides by muSR and NMR

DOI

This proposal describes a muSR experiment on Li-Ti-oxides to see Li diffusion, because muSR is a powerful technique to detect it in the compounds containing magnetic ions. Indeed, according to our preliminary experiment on the positive electrode material LixCoO2, the diffusion constant of Li ions (DLi) estimated by muSR was found to be in good agreement with the prediction of first-principle calculations, while Li-NMR provided considerably lower DLi probably due to the effect of Co 3d spins on the NMR signal. In order to confirm the reliability of DLi estimated by muSR, we wish here to propose a comparative study for Li-Ti-oxides without d electrons, i.e., Li[Li1/3Ti5/3]O4 spinel and Li2TiO3 layered oxide by means of muSR and Li-NMR. Since the two Ti-oxides work as a negative electrode material, the experiment provides essential information on the future solid-state Li-ion batteries.

Identifier
DOI https://doi.org/10.5286/ISIS.E.24075206
Metadata Access https://icatisis.esc.rl.ac.uk/oaipmh/request?verb=GetRecord&metadataPrefix=oai_datacite&identifier=oai:icatisis.esc.rl.ac.uk:inv/24075206
Provenance
Creator Dr Masashi Harada; Dr Jun Sugiyama; Dr Hiroshi Nozaki; Professor Martin Mansson; Dr Izumi Umegaki
Publisher ISIS Neutron and Muon Source
Publication Year 2012
Rights CC-BY Attribution 4.0 International; https://creativecommons.org/licenses/by/4.0/
OpenAccess true
Contact isisdata(at)stfc.ac.uk
Representation
Resource Type Dataset
Discipline Photon- and Neutron Geosciences
Temporal Coverage Begin 2009-09-20T18:00:42Z
Temporal Coverage End 2009-09-22T06:33:05Z