Neutron powder diffraction study of structural and magnetic ground state of the double perovskite seriesLa2-xSrxCuRuO6 (0 <= x <= 1)

DOI

The series of double perovskite oxides La2-xSrxCuRuO6 (0 <= x <= 1) have been reported to have interesting magnetic properties owing to the competing nearest neighbour and next nearest neighbour interactions in combination with the disordered occupancy of Cu and Ru atoms at B/B sites. Full profile refinement of x-ray diffraction patterns predicted a monoclinic structure for the end members while the intermediate members displayed triclinic structure. On the other hand, the parent compound La2CuRuO6 is a short range ferrimagnet while the Sr doped samples clearly display antiferromagnetic ordering at low temperature. The antiferromagnetic ground state of members with lower Sr doping was related to the existence of ferrimagnetic clusters which are antiferromagnetically coupled. In the proposed neutron diffraction experiment we plan to determine the composition dependence of magnetic structure, nature of magnetic interactions and the range of magnetic ordering besides improving the structural information of these fundamentally interesting series of oxides.

Identifier
DOI https://doi.org/10.5291/ILL-DATA.5-31-2277
Metadata Access https://data.ill.fr/openaire/oai?verb=GetRecord&metadataPrefix=oai_datacite&identifier=10.5291/ILL-DATA.5-31-2277
Provenance
Creator Puri, Anil Kumar; Pal, Banabir; Ritter, Clemens; Sarma, Dipankar Das; Roland, Mathieu; Ivanov, Sergey Aleksandrovich; Mukherjee, Sumanta
Publisher Institut Laue-Langevin
Publication Year 2014
Rights OpenAccess; info:eu-repo/semantics/openAccess
OpenAccess true
Representation
Resource Type Dataset
Size 43 MB
Version 1
Discipline Particles, Nuclei and Fields