Investigating the effects of microporous polymer embedded with ionic liquid on CO2 electrolysis in a gas-diffusion electrode for mixed gas r

DOI

Gas-diffusion electrodes (GDEs) modified with a CO₂-philic ionic liquid, [EMIM][BF₄], embedded in a PIM-1 interlayer increase local CO₂ at Ag/Cu catalysts and tolerate impure feeds (N₂/O₂/CO₂ mixture), enabling flue-gas operation without costly purification. Our recent study and ex-situ Raman indicate a specific CO₂–IL interaction. This beamline campaign will (1) provide direct, operando evidence of the role of solid-state [EMIM][BF₄] within PIM-1 and (2) quantify its impact on stability via flooding suppression. We will use GIWAXS (phase/strain; salt/bicarbonate deposits; flooding conditions) under biased, impure-feed conditions, and if possible/needed, XRF to track salt formation (Cs+, K+ ions). Expected outcome: confirmation that the PIM-1+[EMIM][BF₄] layer containing IL, concentrates CO₂, delays water invasion, limits precipitates, and extends steady CO/syngas production on impure streams.

Identifier
DOI https://doi.org/10.15151/ESRF-ES-2437810502
Metadata Access https://icatplus.esrf.fr/oaipmh/request?verb=GetRecord&metadataPrefix=oai_datacite&identifier=oai:icatplus.esrf.fr:inv/2437810502
Provenance
Creator Qiucheng XU ORCID logo; Hesamoddin RABIEE (ORCID: 0000-0003-0439-955X); Alain RIEDER; Xin YU; Lucas WARMUTH (ORCID: 0000-0002-2234-028X); Abhijit DUTTA ORCID logo; Jakub DRNEC ORCID logo
Publisher ESRF (European Synchrotron Radiation Facility)
Publication Year 2029
Rights CC-BY-4.0; https://creativecommons.org/licenses/by/4.0
OpenAccess true
Representation
Resource Type Data from large facility measurement; Collection
Discipline Particles, Nuclei and Fields