With the overall aim of extending the information derivable in a neutron single crystal diffraction experiment beyond the static structure, we are proposing to perform a multi-temperature study of the model system hexamethylenetetramine (HMT) both in the hydrogenated and deuterated form. Two main aspects will be studied: 1) fitting a model potential that include phonons to the diffuse scattering at 300K and 2) perform a full normal mode analysis on data at 10K, 50K, 120K,180K and 250K to benchmark the ability to carry out a similar analysis using powder data from HRPD. The mean square displacements obtained in single crystal diffraction will also be compared to those derived in neutron Compton scattering on VESUVIO.