-
Understanding the spin-Peierls Transition in KTCNQ and derivatives
Motivated by work showing that magnetic coupling between TCNQ anions in potassium TCNQ (KTCNQ) can be changed simply by changing the aromatic substituents, we seek to qunatify... -
Probing the spin dynamics in the pseudo-quaternary Y1-xErxNi2B2C compounds
Our uSR measurements on superconducting Y1-xErxNi2B2C shows a slowing of the Er spin dynamics upon cooling to 2.5 K, but the depolarisation rate does not critically diverge and... -
The search and optimisation of Delta0 resonances in TIPS-Pentacene in solution
To the best of our knowledge, there is no previous work on using muons to measure photo-excited states in organic semiconductors or related materials. Our photo-excitation ideas... -
Detailed temperature dependence of the low-field ALC in TMS-Pentacene
We wish to investigate the evolution of the low-field ALC peaks with temperature of TMS-Pentacene, so we can extract the temperature dependent electron spin relaxation rate. Our... -
characterisation of muonium in functionalized acenes
We wish to measure the high field ALCs of a series of related functionalised acenes, to understand the role of the ligands on the electron spin relaxation, which is of... -
Artificial [FeFe]-Hydrogenases and Muon Spectroscopy
Preliminary measurements of [FeFe]-hydrogenase model complexes were made in a previous experiment using EMU (RB 1010177). The results were interpreted in combination with DFT... -
Muon Spin Relaxation and ALC Resonance in Magnetic and non-Magnetic Oxalate S...
Repolarisation and level crossing resonance will be studied for several different oxalate compounds where muon radical states are known to be formed. Such compounds form a... -
ALC muon spectroscopy of antioxidants
In a previous experiment (RB910492) we have made preliminary measurements of the rates of addition of muonium to vitamins C and E, as suggested by the ISIS panel. These rates... -
Validating a new theoretical method for predicting the HFC of small molecular...
ALC is the best technique to characterize muoniated radicals, that are produced by muonium bonding to unsaturated bonds in molecules. Good agreement between data from ALC and... -
Muon level-crossing resonances as a probe for studying antiferromagnets at pu...
We propose a set of measurements using the HiFi spectrometer in which muon level-crossing resonances are used to probe the internal field inside antiferromagnets in which the... -
Muon spin relaxation studies of KTCNQ and related compounds
Potassium tetracyanoquinodimenthane (KTCNQ) undergoes a spin-Peierls (SP) transition at 396K where a transformation from uniform to dimerised TCNQ- molecules in 1D columns... -
Using muons to investigate the excitation spectrum in low-dimensional molecul...
We propose to use longitudinal field muon-spin relaxation to investigate the excitation spectrum of the most successful realizations of one- and two-dimensional antiferromagnets... -
Understanding the spin-Peierls Transition in KTCNQ and derivatives
Motivated by work showing that magnetic coupling between TCNQ anions in potassium TCNQ (KTCNQ) can be changed simply by changing the aromatic substituents, we seek to qunatify... -
Unconventional superconductivity in quasi-1D K_2Cr_3As_3 (QLCR)
Metallic systems with one-dimensional chain-like atomic structure can support unusual mechanisms for electron pairing leading to superconductivity. K_2Cr_3As_3 is one of a... -
Muon level-crossing resonances as a probe for studying antiferromagnets at pu...
We propose a set of measurements using the HiFi spectrometer in which muon level-crossing resonances are used to probe the internal field inside antiferromagnets in which the... -
Towards a Method of Quantifying Electrophilicity and Nucleophilicity
Understanding of chemical reactivity is founded on the fundamental concepts of Electrophilicity and Neucleophilicity. All extant attempts to do this depend on the reaction of... -
Study of electron spin relaxation in the anthradithiophene series, substitute...
The emerging field of organic spintronics is especially promising for new technologies, owing to the long spin coherence times, large flexibility and low production costs of the... -
Muonium and Flourine Entangled States In An Organic Based Spin Peierls System
Potassium TCNQ is an stoichiometric organic based salt that undergoes a spin Peierls (SP) transition at approximately 390 K. Much research has been conducted on this system in... -
Study of the dependence of electron spin relaxation on molecule length in acenes
We wish to measure the ALCs of a series of polyacene molecules made of a different number of rings. We would like to identify the dependence of the electron spin relaxation rate... -
Utilising Quadrupolar Level Crossing Resonance to Gain Important Information ...
There is much debate about muon stopping sites within materials and in many cases knowing where the muon stops is crucial to understanding the physical properties of different...