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Understanding the spin-Peierls Transition in KTCNQ and derivatives
Motivated by work showing that magnetic coupling between TCNQ anions in potassium TCNQ (KTCNQ) can be changed simply by changing the aromatic substituents, we seek to qunatify... -
Extreme Muon Quantum Effects in Solid Acetone
Extreme muon quantum effects will be studied in the simple organic molecule acetone in deuterated and undeuterated forms using ALC spectroscopy to determine the quantum averaged... -
Probing the spin dynamics in the pseudo-quaternary Y1-xErxNi2B2C compounds
Our uSR measurements on superconducting Y1-xErxNi2B2C shows a slowing of the Er spin dynamics upon cooling to 2.5 K, but the depolarisation rate does not critically diverge and... -
µSR investigation of NaxLi12-xC60
An economy based on hydrogen as an energy carrier is one of the most promising solutions against the greenhouse effect problem, due to the large amount of energy produced by the... -
The search and optimisation of Delta0 resonances in TIPS-Pentacene in solution
To the best of our knowledge, there is no previous work on using muons to measure photo-excited states in organic semiconductors or related materials. Our photo-excitation ideas... -
Detailed temperature dependence of the low-field ALC in TMS-Pentacene
We wish to investigate the evolution of the low-field ALC peaks with temperature of TMS-Pentacene, so we can extract the temperature dependent electron spin relaxation rate. Our... -
characterisation of muonium in functionalized acenes
We wish to measure the high field ALCs of a series of related functionalised acenes, to understand the role of the ligands on the electron spin relaxation, which is of... -
Spin Rotation Experiments at a Pulsed Muon Source using Broadband RF Pulses
In this proposal we wish to explore how the RF-MuSR technique might be developed for measurements akin to FT-NMR. Our work will focus on the broadband excitation of paramagnetic... -
Artificial [FeFe]-Hydrogenases and Muon Spectroscopy
Preliminary measurements of [FeFe]-hydrogenase model complexes were made in a previous experiment using EMU (RB 1010177). The results were interpreted in combination with DFT... -
Quantum spin liquids: beyond Herbertsmithite
We aim at exploring the ground state of new Cu2+ S=1/2 kagome compounds, isomorphic to the now-celebrated Herbertsmithite, namely CdCu3(OH)6Cl2 and MgCu3(OH)6Cl2. Due to the... -
Muon Spin Relaxation and ALC Resonance in Magnetic and non-Magnetic Oxalate S...
Repolarisation and level crossing resonance will be studied for several different oxalate compounds where muon radical states are known to be formed. Such compounds form a... -
Muon level-crossing resonances as a probe for studying antiferromagnets at pu...
We propose a set of measurements using the HiFi spectrometer in which muon level-crossing resonances are used to probe the internal field inside antiferromagnets in which the... -
Hunting for the low-temperature, low-field magnetization plateau in Tb2Ti2O7
Tb2Ti2O7 is a pyrochlore antiferromagnet that has previously been viewed as a spin liquid. This description fails to describe key features of its physics and more recently the... -
Models of the [FeFe]-hydrogenase active site: raising the symmetry
The [FeFe]-hydrogenase enzymes are some of the best catalysts know for generating hydrogen. We have an ongoing programme to understand how their chemistry works, and to... -
Muon spin relaxation studies of KTCNQ and related compounds
Potassium tetracyanoquinodimenthane (KTCNQ) undergoes a spin-Peierls (SP) transition at 396K where a transformation from uniform to dimerised TCNQ- molecules in 1D columns... -
Understanding the spin-Peierls Transition in KTCNQ and derivatives
Motivated by work showing that magnetic coupling between TCNQ anions in potassium TCNQ (KTCNQ) can be changed simply by changing the aromatic substituents, we seek to qunatify... -
Unconventional superconductivity in quasi-1D K_2Cr_3As_3 (QLCR)
Metallic systems with one-dimensional chain-like atomic structure can support unusual mechanisms for electron pairing leading to superconductivity. K_2Cr_3As_3 is one of a... -
Muon level-crossing resonances as a probe for studying antiferromagnets at pu...
We propose a set of measurements using the HiFi spectrometer in which muon level-crossing resonances are used to probe the internal field inside antiferromagnets in which the... -
Microwave µSR studies of solids: electron-hole separation by non-thermal micr...
In this proposal we are planning to study free radicals (molecules with unpaired electrons) and interactions of charged species in solids under microwave irradiation. The study... -
Study of electron spin relaxation in the anthradithiophene series, substitute...
The emerging field of organic spintronics is especially promising for new technologies, owing to the long spin coherence times, large flexibility and low production costs of the...