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Towards a Method of Quantifying Electrophilicity and Nucleophilicity
Understanding of chemical reactivity is founded on the fundamental concepts of Electrophilicity and Neucleophilicity. All extant attempts to do this depend on the reaction of... -
A muSR spectroscopic study of the spin dynamics and reentrant spin-glass tran...
We have recently synthesised the novel iridocuprate IrSr2Sm1.15Ce0.85Cu2O10. This material exhibits a complex temperature dependence of the magnetic susceptibility with multiple... -
Muon level-crossing resonances as a probe for studying antiferromagnets at pu...
We propose a set of measurements using the HiFi spectrometer in which muon level-crossing resonances are used to probe the internal field inside antiferromagnets in which the... -
Kinetics of Hydrogen Abstraction in Alkanes by Mu Reactivity studied by RF Re...
Hydrogen abstraction reactions are key steps in free radical mechanisms that dominate the combustion and atmospheric chemistry of the alkane hydrocarbons and, as such, merit... -
A second generation 2D antiferromagnet investigated with muons
Low-dimensional quantum magnetism continues to be of great theoretical and experimental interest, as reduced dimensionality supports strong quantum fluctuations which can result... -
Oxygen deficiency in the quantum spin ice Tb2Ti2O7
Tb2Ti2O7 is one of two compounds identified as potential quantum spin ices. As with other oxide pyrochlores the properties depend sensitively on the oxygen content. Most... -
Muon States in Nanostructured Carbonaceous Materials
This experiment proposes the continuation of a study, initiated at J-PARC, on a new type of activated carbon material, with a pore structure and chemistry "tunable" in a manner... -
RF MuSR in the gas phase: The Search for a Radical State (RB920227)
The main spectroscopic technique for studying radicals in solids and liquids, ESR, cannot usually be used to study radicals of more than 3-5 atoms in the gas phase due to strong... -
Unconventional superconductivity in quasi-1D K_2Cr_3As_3 (QLCR)
Metallic systems with one-dimensional chain-like atomic structure can support unusual mechanisms for electron pairing leading to superconductivity. K_2Cr_3As_3 is one of a... -
Muon spin relaxation studies of KTCNQ and related compounds
Potassium tetracyanoquinodimenthane (KTCNQ) undergoes a spin-Peierls (SP) transition at 396K where a transformation from uniform to dimerised TCNQ- molecules in 1D columns... -
Kinetics of Hydrogen Abstraction in Alkanes by Mu Reactivity studied by RF Re...
Hydrogen abstraction reactions are key steps in free radical mechanisms that dominate the combustion and atmospheric chemistry of the alkane hydrocarbons and, as such, merit... -
RF MuSR in the gas phase: The Search for a Radical State
The main spectroscopic technique for studying radicals in solids and liquids, ESR, cannot usually be used to study radicals of more than 3-5 atoms in the gas phase due to strong... -
Hunting for the low-temperature, low-field magnetization plateau in Tb2Ti2O7
Tb2Ti2O7 is a pyrochlore antiferromagnet that has previously been viewed as a spin liquid. This description fails to describe key features of its physics and more recently the... -
Muon level-crossing resonances as a probe for studying antiferromagnets at pu...
We propose a set of measurements using the HiFi spectrometer in which muon level-crossing resonances are used to probe the internal field inside antiferromagnets in which the... -
Repolarization of Radicals in Liquids
The recovery of the muon polarization in a longitudinal magnetic field has been used to obtain the muon hfcs of organic radicals. In pure benzene there is a single step in the... -
Muon Spin Relaxation and ALC Resonance in Magnetic and non-Magnetic Oxalate S...
Repolarisation and level crossing resonance will be studied for several different oxalate compounds where muon radical states are known to be formed. Such compounds form a... -
Spin fluctuations in heavy fermion system
A study of the ground state of the Ce5Rh4Sn10 is proposed. Compound belongs to the heavy fermion system with two magnetic phase transitions at 1.4 K and 4.3 K. While the... -
Artificial [FeFe]-Hydrogenases and Muon Spectroscopy
Preliminary measurements of [FeFe]-hydrogenase model complexes were made in a previous experiment using EMU (RB 1010177). The results were interpreted in combination with DFT... -
characterisation of muonium in functionalized acenes
We wish to measure the high field ALCs of a series of related functionalised acenes, to understand the role of the ligands on the electron spin relaxation, which is of... -
Muonium in cubic stabilized zirconia
This proposal is part of a long-range program aiming at determining the stable charge-stateconfigurations, site and impurity energy levels (donor and/or acceptor) of hydrogen in...