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Frustration, quantum spin ices and quantum diffusion
This proposal aims to characterise the spin dynamics of three Pr-based pyrochlores that may be realisations of quantum spin ice materials. The lower moment and larger wave... -
DYNAMICS OF SURFACTANTS IN LUBRICATING OILS
In a recent series of successful experiments at PSI and ISIS we were able to demonstrate the possibility of measuring the rate of transfer of a small molecule (allyl alcohol)... -
Oxygen deficiency in the quantum spin ice Tb2Ti2O7
Tb2Ti2O7 is one of two compounds identified as potential quantum spin ices. As with other oxide pyrochlores the properties depend sensitively on the oxygen content. Most... -
Magnetic ionic liquid surfactants
This proposal is to explore the magnetic properties and molecular dynamics of a new class of magnetic ionic liquid surfactants1 (MILSs) (see Fig. 1). The MILSs investigated here... -
Spin Rotation Experiments at a Pulsed Muon Source using Broadband RF Pulses
In this proposal we wish to explore how the RF-MuSR technique might be developed for measurements akin to FT-NMR. Our work will focus on the broadband excitation of paramagnetic... -
Muon Spin Relaxation studies of Ni2TCNQ, Ni(TCNQ)2 and related materials
Amorphous molecular magnetic materials Ni2(OA) (OA:organic acceptor) were reported to exhibit ferromagnetism with Curie temperatures >400K. This work is controversial as it... -
muSR in the presence of significant spin-orbit coupling
The great majority of known muonium defect centres and muonium substituted organic radicals have essentially spin-only magnetism, with few exhibiting any noticeable departure... -
Muonium in alpha-boron
Previous muon experiments have identified a muonium state in the commonly occuring, but complex, beta rhombohedral form of elemental boron. To complement recent theoretical work... -
Investigation of carrier transport in the organic semiconductor 8-hydroxy-qui...
Using the Emu spectrometer at ISIS we have recently studied charge carrier transport in the technologically important molecule 8-hydroxy-quinoline aluminium, by probing the... -
Repolarization of Radicals in Liquids (RB920344)
The recovery of the muon polarization in a longitudinal magnetic field has been used to obtain the muon hfcs of organic radicals. In pure benzene there is a single step in the... -
Spin-lattice relaxation in holmium-based high symmetry single-molecule magnets
The study of spin-lattice relaxation in mononuclear lanthanide complexes is justified by the potential applications of these so-called single-molecule magnets in quantum... -
Multiferroicity in metal-formate perovskites
Recent work has revealed that metal-organic frameworks (MOFs) can also exhibit this multiferroicity. These materials are particularly interesting since their structures are... -
End-Game: Cornering Solvent Effects on H-Addition in Green Tea Anti-Oxidants
Our ongoing project to characterise radical scavenging by the green tea anti-oxidant EGCG and its D-ring analogue, (3,4,5-(OH)3-Bz) is near-complete. ALC-MuSR experiments on the... -
Hydrogen impurity in solar cell materials CIGS and CZTS
In this proposal we intend to complete the characterization of the hydrogen impurity in solar cell materials Cu2ZnSnS4 (CZTS) and Cu(In,Ga)Se2 (CIGS), by using the positive... -
Identifying the mechanism behind spin relaxation in organic materials
We wish to measure the low-field ALCs of a series of related functionalised acenes to identify which mechanism (spin orbit or hyperfine) is responsible for spin relaxation in... -
Utilising Quadrupolar Level Crossing Resonance to Gain Important Information ...
There is much debate about muon stopping sites within materials and in many cases knowing where the muon stops is crucial to understanding the physical properties of different... -
Muonium in widegap oxides
This proposal is part of a long-range program aiming at determining the stable charge-state configurations, site and impurity energy levels (donor and/or acceptor) of hydrogen... -
Development of Radio Frequency µSR as a Method for Determining Hyperfine Coup...
Radio Frequency µSR provides a direct method for accurately determining muon hyperfine coupling constants, Aµ, for muoniated radical species. The method complements the well... -
Dynamics in a new skyrmion spin texture in GaV4S8
Topological physics was the subject of this year's Nobel Prize for Physics and over forty years after the groundbreaking work of Kosterlitz, Thouless and Haldane, remains an... -
Probing the [FeFe]-hydrogenase subsite using muon spectroscopy
Solid state repolarisation measurements of [Fe2(µ-pdt)(CO)4(PMe3)2] (RB 1010177) showed a weak recovery at ca.15G, a strong recovery at ca.100G and what was thought to be a weak...