Operando Studies of Anion Intercalation into Graphite Cathodes of Aluminium Graphite Batteries

DOI

Aluminium carbon battery is an emerging battery technology based on aluminium anodes and cathodes made from carbon /graphite. The materials are abundant, and the production of these batteries might be even simpler than today’s Li-ion batteries (depending on the electrolyte). The charge-discharge mechanism is based on deposition and stripping of aluminium on the anode, while anions from the electrolyte are intercalating into the carbon cathode. The most commonly employed electrolyte is based on the AlCl3 salt dissolved in the ionic liquid EmimCl. The active anion with respect to the cathode intercalation reaction is normally claimed to be AlCl4-, even if the size of this anion is much larger than the interlayer spacing of graphite. In addition, side reactions (partly reversible) lead to the formation of surface products that might be crystalline in nature. Operando X-ray diffraction studies are therefore well suited for improved understanding of this intercalation reaction.

Identifier
DOI https://doi.org/10.15151/ESRF-ES-2439530278
Metadata Access https://icatplus.esrf.fr/oaipmh/request?verb=GetRecord&metadataPrefix=oai_datacite&identifier=oai:icatplus.esrf.fr:inv/2439530278
Provenance
Creator Anders GAARUD ORCID logo; Maria Valeria BLANCO ORCID logo; Ann Mari SVENSSON ORCID logo; Helene Lillevestre LANGLI; Dmitry CHERNYSHOV
Publisher ESRF (European Synchrotron Radiation Facility)
Publication Year 2029
Rights CC-BY-4.0; https://creativecommons.org/licenses/by/4.0
OpenAccess true
Representation
Resource Type Data from large facility measurement; Collection
Discipline Particles, Nuclei and Fields