In-situ nano-tomography on nano-porous silicon particles for lithium-ion batteries.

DOI

Silicon (Si) is the most promising anode material to increase lithium ion battery energy density. This performance is due in part to the large amount of lithium it can alloy with. However, that amount of (de)lithiation leads to the expansion (or contraction) of particles up to 280%, which induces mechanical degradation at many electrode levels. Our strategy is to buffer this volume expansion with Si particles containing inner porosity. But, it works if the latter is preserved, which is very difficult to assess in working battery conditions. Here we will use X-ray nano-tomography to monitor the Si particles morphological changes down to the nano-scale, as well as possible electrode degradation during cycling (in situ conditions). This will provide unprecedented insight in the role of porosity, providing direction to porous silicon development for the next generation of high energy density batteries. This proposal involves an industrial partner: E-magy, who provides the Si electrodes.

Identifier
DOI https://doi.org/10.15151/ESRF-ES-2438147344
Metadata Access https://icatplus.esrf.fr/oaipmh/request?verb=GetRecord&metadataPrefix=oai_datacite&identifier=oai:icatplus.esrf.fr:inv/2438147344
Provenance
Creator Lucas HUET ORCID logo; SANDRINE LYONNARD ORCID logo; Julie VILLANOVA; Marceau VIORNERY; Riwan ABDELKHALIK; XAVER SIMON BREMS ORCID logo; Pranav KARANTH ORCID logo; Wenxuan ZHAO ORCID logo; Victor VANPEENE (ORCID: 0000-0002-5383-440X); MRINALINI CHATTERJEE ORCID logo; Swapna GANAPATHY ORCID logo
Publisher ESRF (European Synchrotron Radiation Facility)
Publication Year 2029
Rights CC-BY-4.0; https://creativecommons.org/licenses/by/4.0
OpenAccess true
Representation
Resource Type Data from large facility measurement; Collection
Discipline Particles, Nuclei and Fields