Applying XAS to uncover electron-deficiency multicenter bonding in SnxChy chalcogenides (Ch = 0, S, Se, Te) subjected to high pressure

DOI

Electron-deficiency multicenter bonding (EDMB) has been proposed as an incipient, novel chemical bond behind the outstanding properties of promising materials as phase change materials, thermoelectrics, photovoltaic materials and topological insulators. High pressure (HP) can easily induced such EDMB in systems with stereochemically active lone electron pairs (SCALEPs). As we have evidenced for the mixed-valence Sn2S3, XAS has been proved to be an essential technique to unveil these EDMBs, in addition to single-crystal XRD and Raman spectroscopy under HP. This project aims to demonstrate how XAS can be used the emergence of these bonds in other Sn-based chalcogenides. Then, we propose to collect Sn K-edge XAS measurements on SnTe (without SCALEPs), SnSe and Sn3O4 (both with SCALEPs) under HP, up to 50 GPa, to undoubtedly propose the XAS technique as alternative tool to follow the emergence of EDMBs

Identifier
DOI https://doi.org/10.15151/ESRF-ES-2170279797
Metadata Access https://icatplus.esrf.fr/oaipmh/request?verb=GetRecord&metadataPrefix=oai_datacite&identifier=oai:icatplus.esrf.fr:inv/2170279797
Provenance
Creator Samuel GALLEGO PARRA ORCID logo; Yimin MIJITI ORCID logo; Marina CANDELA DE AROCA ORCID logo
Publisher ESRF (European Synchrotron Radiation Facility)
Publication Year 2028
Rights CC-BY-4.0; https://creativecommons.org/licenses/by/4.0
OpenAccess true
Representation
Resource Type Data from large facility measurement; Collection
Discipline Particles, Nuclei and Fields