Materials with magnetic interactions between their metal centres play a tremendous role in modern technologies and can exhibit unique physical phenomena. The inability of traditional magnetic compounds to realise optimal material parameters or embody model hamiltonians has resulted in attention being turned to metal-organic frameworks (MOFs), which present a versatile platform for the realization of complex magnets due to their molecular building-block nature. (Me2NH2)2[Fe2L3]·2H2O·6DMF Is a novel system with Fe(III) ions in a perfect honeycomb lattice, where in-situ reduction of the ligands increases Tc from 80 to 150K, whilst preserving the crystallinity and structure. We wish to investigate the magnetic excitations of the Fe compound, and we will also synthesise a Ru(III) analogue and measure it in addition. This is combined with another proposal studying the magnetic structure.