Antiplasticizing effect of water in amorphous prilocaine

DOI

In glassforming organic materials, the addition of water usually has a direct plasticizing effect, visible in a lowering of the glass-transition temperature Tg upon hydration of the material (the lower the Tg the higher the relative water content). We have observed an antiplasticizing effect in a small molecule, prilocaine, caused by the addition of water. This shift in Tg has been observed both with Differential Scanning Calorimetry experiments and Broadband Dielectric Spectroscopy. The microscopic hydrating mechanisms underlying the macroscopic antiplasticizing effect upon the addition of water to prilocaine are still unknown. Here we propose to investigate the hydration structure of prilocaine in solution using neutron diffraction coupled with both EPSR and Molecular dynamics simulations.

Identifier
DOI https://doi.org/10.5286/ISIS.E.86387911
Metadata Access https://icatisis.esc.rl.ac.uk/oaipmh/request?verb=GetRecord&metadataPrefix=oai_datacite&identifier=oai:icatisis.esc.rl.ac.uk:inv/86387911
Provenance
Creator Dr Silvia Imberti; Ms Guadalupe Ruiz; Dr Sylvia McLain; Ms Nicola Steinke; Dr Luis Carlos Pardo-Soto; Dr Silvina Cerveny; Dr Michela Romanini; Dr Jose Luis Tamarit; Dr Roberto Macovez
Publisher ISIS Neutron and Muon Source
Publication Year 2020
Rights CC-BY Attribution 4.0 International; https://creativecommons.org/licenses/by/4.0/
OpenAccess true
Contact isisdata(at)stfc.ac.uk
Representation
Resource Type Dataset
Discipline Chemistry; Natural Sciences; Physics
Temporal Coverage Begin 2017-05-25T08:00:00Z
Temporal Coverage End 2017-05-28T20:01:08Z