Li-induced Stress Distributions in Si Thin Films with Chevron-like Nanostructures

DOI

Silicon is one of the most promising anode materials in solid-state batteries due to its very high specific capacity. Current results are however still in an infant state in terms of electrochemical performance, analytical characterization and mechanistic understanding. During lithiation/delithation, Si undergoes a substantial ∼300 % volume change, can lead to structural damage. The underlying electro-chemo-mechanical behavior of Si anodes remains so far inadequately understood and validating theoretical models has proven to be a challenging task. The objective is to precisely quantify the evolution of cross-sectional stress distributions in thin Si films with varying grain boundary morphology during lithiation and delithiation processes. To achieve this, we will employ cross-sectional X-ray nanodiffraction to characterize Si and LixSi phases. The experiment will reveal, how the chevron-like nanostructure of the films correlate with the observed electro-chemo-mechanical behavior.

Identifier
DOI https://doi.org/10.15151/ESRF-ES-1703086548
Metadata Access https://icatplus.esrf.fr/oaipmh/request?verb=GetRecord&metadataPrefix=oai_datacite&identifier=oai:icatplus.esrf.fr:inv/1703086548
Provenance
Creator Francois LIENARD (ORCID: 0000-0001-6825-454X); Atacan ASCI ORCID logo; Henrik ROTVÆR BRATLIE; Jozef KECKES; Michael MEINDLHUMER ORCID logo; QUOC HUNG NGUYEN ORCID logo; Juraj TODT (ORCID: 0000-0003-3067-798X); Isabella SILVA BARRETO ORCID logo
Publisher ESRF (European Synchrotron Radiation Facility)
Publication Year 2027
Rights CC-BY-4.0; https://creativecommons.org/licenses/by/4.0
OpenAccess true
Representation
Resource Type Data from large facility measurement; Collection
Discipline Particles, Nuclei and Fields