Low dimensional networks under pressure. In-situ diffraction measurements of carbonate glasses.

DOI

Carbonate liquids are characterised by low temperature and low viscosity and play an important role in molten carbonate fuel cells, battery electrolytes and, surprisingly, in volcanic processes. Indeed they are important agents of element transfer in the deep Earth interior. Despite their unique role determined by structure-related properties little is known about the carbonate liquid structure. The aim of this work is to determine what happens to the carbonate chains when pressure is applied. We have recently completed an experiment on carbonate glasses at 3.3 and 8.5GPa. Ultrasonic measurements suggest a sudden change in the sound velocity in this region and in this proposal we will further explore this regime where structures change most by collected diffraction data for a pressure point at 6GPa. This will be augmented by simulation and NMR measurements.

Identifier
DOI https://doi.org/10.5286/ISIS.E.84782836
Metadata Access https://icatisis.esc.rl.ac.uk/oaipmh/request?verb=GetRecord&metadataPrefix=oai_datacite&identifier=oai:icatisis.esc.rl.ac.uk:inv/84782836
Provenance
Creator Dr Martin Wilding; Dr Craig Bull
Publisher ISIS Neutron and Muon Source
Publication Year 2020
Rights CC-BY Attribution 4.0 International; https://creativecommons.org/licenses/by/4.0/
OpenAccess true
Contact isisdata(at)stfc.ac.uk
Representation
Resource Type Dataset
Discipline Natural Sciences; Physics
Temporal Coverage Begin 2017-03-04T10:00:00Z
Temporal Coverage End 2017-03-07T10:00:00Z