Engineering epitaxial interfaces for topological insulator – superconductor hybrid devices with Al electrodes

DOI

Proximity-induced superconductivity in hybrid devices of topological insulators and superconductors offers a promising platform for the pursuit of elusive topological superconductivity and its anticipated applications, such as fault-tolerant quantum computing. To study and harness such hybrid devices, a key challenge is the realization of highly functional material interfaces with a suitable superconductor featuring 2e-periodic parity-conserving transport to ensure a superconducting hard-gap free of unpaired electrons, which is important for Majorana physics. A superconductor well-known for this characteristic is Al, however, its direct integration into devices based on tetradymite topological insulators has so far been found to yield non-transparent interfaces. By focusing on Bi₂Te₃-Al heterostructures, this study identifies detrimental interdiffusion processes at the interface through atomically resolved structural and chemical analysis, and showcase their mitigation by leveraging different interlayers – namely Nb, Ti, Pd, and Pt – between Bi₂Te₃ and Al. Through structural transformation of the interlayer materials (X) into their respective tellurides (XTe₂) atomically-sharp epitaxial interfaces are engineered and further characterized in low-temperature transport experiments on Al-X-Bi₂Te₃-X-Al Josephson junctions and in complementary density functional theory calculations. By demonstrating functional interfaces between Bi₂Te₃ and Al, this work provides key insights and paves the way for the next generation of sophisticated topological devices.

Identifier
DOI https://doi.org/10.24435/materialscloud:w3-3c
Related Identifier https://doi.org/10.5281/zenodo.3628251
Related Identifier https://doi.org/10.1038/s41524-020-00482-5
Related Identifier https://doi.org/10.5281/zenodo.7284739
Related Identifier https://doi.org/10.1103/PhysRevB.105.125143
Related Identifier https://doi.org/10.5281/zenodo.7576163
Related Identifier https://renkulab.io/projects/new?data=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
Related Identifier https://archive.materialscloud.org/communities/mcarchive
Related Identifier https://doi.org/10.24435/materialscloud:m1-7c
Metadata Access https://archive.materialscloud.org/oai2d?verb=GetRecord&metadataPrefix=oai_dc&identifier=oai:materialscloud.org:2360
Provenance
Creator Jalil, Abdur Rehman; Schmitt, Tobias W.; Rüßmann, Philipp; Wei, Xian-Kui; Frohn, Benedikt; Schleenvoigt, Michael; Wittl, Wilhelm; Hou, Xiao; Schmidt, Anne; Underwood, Kaycee; Bihlmayer, Gustav; Luysberg, Martina; Mayer, Joachim; Blügel, Stefan; Grützmacher, Detlev; Schüffelgen, Peter
Publisher Materials Cloud
Contributor Jalil, Abdur Rehman; Rüßmann, Philipp
Publication Year 2024
Rights info:eu-repo/semantics/openAccess; Creative Commons Attribution 4.0 International; https://creativecommons.org/licenses/by/4.0/legalcode
OpenAccess true
Contact archive(at)materialscloud.org
Representation
Language English
Resource Type info:eu-repo/semantics/other
Format application/octet-stream; text/markdown; text/plain; application/prs.xsf+xml; application/zip; text/x-python
Discipline Materials Science and Engineering