Engineering epitaxial interfaces for topological insulator – superconductor hybrid devices with Al electrodes

Proximity-induced superconductivity in hybrid devices of topological insulators and superconductors offers a promising platform for the pursuit of elusive topological superconductivity and its anticipated applications, such as fault-tolerant quantum computing. To study and harness such hybrid devices, a key challenge is the realization of highly functional material interfaces with a suitable superconductor featuring 2e-periodic parity-conserving transport to ensure a superconducting hard-gap free of unpaired electrons, which is important for Majorana physics. A superconductor well-known for this characteristic is Al, however, its direct integration into devices based on tetradymite topological insulators has so far been found to yield non-transparent interfaces. By focusing on Bi₂Te₃-Al heterostructures, this study identifies detrimental interdiffusion processes at the interface through atomically resolved structural and chemical analysis, and showcase their mitigation by leveraging different interlayers – namely Nb, Ti, Pd, and Pt – between Bi₂Te₃ and Al. Through structural transformation of the interlayer materials (X) into their respective tellurides (XTe₂) atomically-sharp epitaxial interfaces are engineered and further characterized in low-temperature transport experiments on Al-X-Bi₂Te₃-X-Al Josephson junctions and in complementary density functional theory calculations. By demonstrating functional interfaces between Bi₂Te₃ and Al, this work provides key insights and paves the way for the next generation of sophisticated topological devices.

Identifier
Source https://archive.materialscloud.org/record/2024.174
Metadata Access https://archive.materialscloud.org/xml?verb=GetRecord&metadataPrefix=oai_dc&identifier=oai:materialscloud.org:2360
Provenance
Creator Jalil, Abdur Rehman; Schmitt, Tobias W.; Rüßmann, Philipp; Wei, Xian-Kui; Frohn, Benedikt; Schleenvoigt, Michael; Wittl, Wilhelm; Hou, Xiao; Schmidt, Anne; Underwood, Kaycee; Bihlmayer, Gustav; Luysberg, Martina; Mayer, Joachim; Blügel, Stefan; Grützmacher, Detlev; Schüffelgen, Peter
Publisher Materials Cloud
Publication Year 2024
Rights info:eu-repo/semantics/openAccess; Creative Commons Attribution 4.0 International https://creativecommons.org/licenses/by/4.0/legalcode
OpenAccess true
Contact archive(at)materialscloud.org
Representation
Language English
Resource Type Dataset
Discipline Materials Science and Engineering