Bridging Indoor and Outdoor Perovskite Degradation Using Physics Modeling and Bayesian Analysis

DOI

In this work, we use physics-based modelling with a probabilistic Bayesian framework, relying solely on current-density-voltage (J-V) curves recorded throughout aging in both indoor and outdoor degradation tests. We investigate whether the same degradation mechanisms occur in both outdoor tests and indoor accelerated aging tests — an important step toward identifying the dominant degradation mechanisms from commonly available data and establishing the validity of accelerated aging tests. The data provided here includes these J-V curves as well as the outdoor maximum power point tracking (MPPT) data with corresponding irradiance and cell temperature recordings. For the indoor accelerated tests, the J-V curves were recorded during the aging process and therefore under the same aging conditions of the cells: ~1.3 suns and fixed temperature levels (25, 45, 65 and 85 °C). The aging setup and measurement routine were detailed in Köbler (2022). The indoor_jvs.csv file includes the following information: cell_id: such as D1_P1, represents substrate 1 (D1), cell 1 (P1), where each substrate contains six electrically isolated perovskite solar cells. Note that the naming of substrates restarts at each temperature; temp: the aging temperature in °C; meas_time: the time in hours since the start of aging; scan: scan direction of J-V (FOR: forward; REV: reverse); v and j: the raw voltage and current density data (as lists). For the outdoor tests, J-V curves were recorded under a sun simulator at standard test conditions (1 sun, 25 °C). The outdoor_jvs.csv file follows the same structure as the indoor data, with two exceptions: the temp column is omitted, and meas_time is given as a date. The outdoor MPPT data (outdoor_mpp_) is provided separately for three cells and includes voltage, current, and power at MPP as a timeseries. Irradiance and cell temperature data are provided in a separate merged file (irradiance_and_cell_temp.csv).

Identifier
DOI https://doi.org/10.5442/ND000013
Related Identifier Cites https://doi.org/10.1002/ente.202200234
Related Identifier IsSupplementTo https://doi.org/10.1002/solr.202500716
Metadata Access https://data.helmholtz-berlin.de/oaipmh/request?verb=GetRecord&metadataPrefix=oai_datacite&identifier=oai:data.helmholtz-berlin.de:datapub/13
Provenance
Creator Chakar, Joseph; Erdil, Ulas ORCID logo; Burgaud, Antoine; Remec, Marko (ORCID: 0000-0002-4246-364X); Abate, Antonio ORCID logo; Ulbrich, Carolin ORCID logo; Schlatmann, Rutger ORCID logo; Bonnassieux, Yvan; Khenkin, Mark ORCID logo; Puel, Jean-Baptiste
Publisher HZB Data Service
Publication Year 2025
Rights Creative Commons Zero v1.0 Universal; https://creativecommons.org/publicdomain/zero/1.0/
OpenAccess true
Representation
Resource Type Dataset
Format text/csv
Size 286.99 MiB
Discipline Other