Elucidation of oxygen-redox charge-compensation mechanism for Na-ion battery O3-type cathode Na1Li1/3Mn2/3O2 by operando O K-edge XAS enable

DOI

A new experiment is proposed for operando acquisition of O K-edge XAS spectra through XRS for sodium-ion battery (SIB) cathode. This would be the first experiment suitable for operando investigation of oxygen-redox behaviour, where we can distinguish the formation of the different oxidized O-species in the corresponding potential windows. We expect that it will specifically support or disprove the current theory on oxygen-redox-active sodium¬¬¬-manganese¬ layered oxides. However, in principle, this experiment also will provide evidence for reaching a unified understanding of oxygen-redox processes in any oxygen-redox-active materials and therefore is of high interest for the whole rechargeable battery community.

Identifier
DOI https://doi.org/10.15151/ESRF-ES-2104246899
Metadata Access https://icatplus.esrf.fr/oaipmh/request?verb=GetRecord&metadataPrefix=oai_datacite&identifier=oai:icatplus.esrf.fr:inv/2104246899
Provenance
Creator Christoph SAHLE ORCID logo; Renier ARABOLLA RODRIGUEZ; Samuel GATTI; Łukasz KONDRACKI
Publisher ESRF (European Synchrotron Radiation Facility)
Publication Year 2028
Rights CC-BY-4.0; https://creativecommons.org/licenses/by/4.0
OpenAccess true
Representation
Resource Type Data from large facility measurement; Collection
Discipline Particles, Nuclei and Fields