Atomic structure of mercury chalcohalide glasses

DOI

Optical applications of chalcogenide glasses need a wide transparency window in far IR. Promising glass systems include HgI2. We have synthesised three vitreous systems yHgI2.(1-y)As2X3, where X = S, Se, Te. The max HgI2 content in the glass increases with atomic number from y = 0.2 (S) to y = 0.8 (Te). In order to decode the structure of these exciting new glasses and to understand an enormous difference in their glass-forming ability, we are planning ND measurements of 8 glasses in the 3 systems. Our recent feasibility experiment using GEM has shown that we are able to obtain a high-quality data on these strongly absorbing samples. In particular, the y = 0.2 sulphide glass seems to contain mercury iodide in a molecular form. This is the first direct structural information on mercury environment in a chalcohalide glass.

Identifier
DOI https://doi.org/10.5286/ISIS.E.42592996
Metadata Access https://icatisis.esc.rl.ac.uk/oaipmh/request?verb=GetRecord&metadataPrefix=oai_datacite&identifier=oai:icatisis.esc.rl.ac.uk:inv/42592996
Provenance
Creator Professor Eugene Bychkov; Dr Mariana Milochova; Dr Alex Hannon
Publisher ISIS Neutron and Muon Source
Publication Year 2016
Rights CC-BY Attribution 4.0 International; https://creativecommons.org/licenses/by/4.0/
OpenAccess true
Contact isisdata(at)stfc.ac.uk
Representation
Resource Type Dataset
Discipline Photon- and Neutron Geosciences
Temporal Coverage Begin 2013-09-30T12:18:56Z
Temporal Coverage End 2013-10-04T15:12:52Z