Investigating regiochemistry of artificial [FeFe]-hydrogenase subsites using muon spectroscopy

DOI

During our recent experiment (RB1310434) we were able to use ALC to characterise the radical states formed in [Fe2(µ-pdt)(CO)4(PMe3)2] and [Fe2(µ-pdt)(CO)4(CN)2]2- at two temperatures. The ALC spectra of [Fe2(µ-pdt)(CO)4(PMe3)2] displays a feature, the broadness and position shows temperature dependence. The broadness of this feature is consistent with the multiple binding sites predicted by the DFT calculations with couplings in the range ~200-300MHz. We propose investigating the evolution of the ALC lineshape as a function of temperature. The ALC spectra of [Fe2(µ-pdt)(CO)4(CN)2]2- shows a triplet of features between ca.12,000G and ca.16,000G, the positions of which are also temperature dependant. We would like to study these resonances as a function of temperature using high statistics.

Identifier
DOI https://doi.org/10.5286/ISIS.E.24091211
Metadata Access https://icatisis.esc.rl.ac.uk/oaipmh/request?verb=GetRecord&metadataPrefix=oai_datacite&identifier=oai:icatisis.esc.rl.ac.uk:inv/24091211
Provenance
Creator Dr Stephen Cottrell; Dr Jamie Peck; Dr Joseph Wright; Professor C J Pickett; Dr Upali Jayasooriya; Miss Ausra Jablonskyte
Publisher ISIS Neutron and Muon Source
Publication Year 2016
Rights CC-BY Attribution 4.0 International; https://creativecommons.org/licenses/by/4.0/
OpenAccess true
Contact isisdata(at)stfc.ac.uk
Representation
Resource Type Dataset
Discipline Photon- and Neutron Geosciences
Temporal Coverage Begin 2013-10-24T23:00:00Z
Temporal Coverage End 2013-10-31T00:00:00Z