Methane hydrate formation in the presence of silica nanospheres

DOI

In this Rapid Access request we wish to study in situ formation of methane hydrates in the presence of weakly hydrophilic silica nanospheres. The aim of this research is to enable us to understand and control heterogeneous nucleation at the solid-liquid interface. Urgency stems from recent simulations that have predicted that under the conditions of study, methane, and therefore hydrate, should prefer the bulk to interfacial region. Neutrons and NIMROD are essential for this work, as they will allow us probe the relevant length and timescales, and also to exploit H/D labelling of the methane. In our previously awarded experiment RB1320495 we have successfully studied systems containing planar clay minerals. In this experiment we will study methane hydrate formation in the presence of 20 nm and 100 nm silica nanospheres. This work is part of a BP funded programme ending in December 2014.

Identifier
DOI https://doi.org/10.5286/ISIS.E.54808485
Metadata Access https://icatisis.esc.rl.ac.uk/oaipmh/request?verb=GetRecord&metadataPrefix=oai_datacite&identifier=oai:icatisis.esc.rl.ac.uk:inv/54808485
Provenance
Creator Mr Matt Billing; Dr Diana Taylor; Dr Angelos Michaelides; Dr Neal Skipper; Miss Radhika Patel; Mr Mitch Watts
Publisher ISIS Neutron and Muon Source
Publication Year 2017
Rights CC-BY Attribution 4.0 International; https://creativecommons.org/licenses/by/4.0/
OpenAccess true
Contact isisdata(at)stfc.ac.uk
Representation
Resource Type Dataset
Discipline Construction Engineering and Architecture; Engineering; Engineering Sciences; Natural Sciences; Physics
Temporal Coverage Begin 2014-08-10T23:00:00Z
Temporal Coverage End 2014-08-17T23:00:00Z