Using XRS to probe speciation of lithium cations for battery electrolytes

DOI

Lithium-ion batteries already play a crucial role in energy storage, but there is still plenty of room for improvement in performance. There is a lack of knowledge about the structure of the solvent/anions around the Li+ in solution, mainly due to a lack of available techniques to study Li+ speciation. We propose to overcome this challenge by using X-ray Raman scattering (XRS) at the Li K edge at ID20 to validate our calculations, from which we will then be able to identify the coordination number around Li+ in solution. We will study a wide variety of electrolytes, allowing us to demonstrate that our approach is viable for both already commonly used electrolytes (e.g. Li[PF6] in carbonate solvents) and novel electrolytes that have the potential to overcome some traditional problems with commonly used electrolytes (e.g. ionic liquids).

Identifier
DOI https://doi.org/10.15151/ESRF-ES-2064083681
Metadata Access https://icatplus.esrf.fr/oaipmh/request?verb=GetRecord&metadataPrefix=oai_datacite&identifier=oai:icatplus.esrf.fr:inv/2064083681
Provenance
Creator Christoph SAHLE ORCID logo; Frances TOWERS TOMPKINS; Lewis PARKER ORCID logo; Luke HIGGINS ORCID logo; Kevin LOVELOCK (ORCID: 0000-0003-1431-269X); Blanka DETLEFS (ORCID: 0000-0002-9768-647X)
Publisher ESRF (European Synchrotron Radiation Facility)
Publication Year 2028
Rights CC-BY-4.0; https://creativecommons.org/licenses/by/4.0
OpenAccess true
Representation
Resource Type Data from large facility measurement; Collection
Discipline Particles, Nuclei and Fields