Paramagnetic half-moon shaped diffuse scattering arising from 3D magnetic frustration

DOI

We use spin dynamics simulations to determine the origin of the unusual correlated diffuse scattering, characterised by half-moon shapes bridging the magnetic Bragg peaks, observed in the polarised elastic neutron scattering from manganese tungstate, MnWO₄. We first fit a Heisenberg Hamiltonian with twelve nearest-neighbour exchange interactions and single-ion anisotropy to the experimental ground-state magnon dispersion. We then show via spin dynamics simulations that our model Hamiltonian both reproduces the experimentally observed half-moon features and captures their persistence into the paramagnetic regime. Moreover, we identify the three-dimensional, competing antiferromagnetic interactions driving this behavior. Our work complements earlier studies of half-moon-shaped signatures in pyrochlore and triangular structures, by providing insight into their origin in a zigzag chain geometry with three-dimensional competing exchange interactions.

Identifier
DOI https://doi.org/10.24435/materialscloud:kp-8f
Related Identifier https://doi.org/10.48550/arXiv.2503.23704
Related Identifier https://archive.materialscloud.org/communities/mcarchive
Related Identifier https://doi.org/10.24435/materialscloud:te-81
Metadata Access https://archive.materialscloud.org/oai2d?verb=GetRecord&metadataPrefix=oai_dc&identifier=oai:materialscloud.org:2662
Provenance
Creator Natsch, Nelly; Tošić, Tara; Soh, Jian-Rui; Spaldin, Nicola
Publisher Materials Cloud
Contributor Natsch, Nelly
Publication Year 2025
Rights info:eu-repo/semantics/openAccess; Creative Commons Attribution 4.0 International; https://creativecommons.org/licenses/by/4.0/legalcode
OpenAccess true
Contact archive(at)materialscloud.org
Representation
Language English
Resource Type info:eu-repo/semantics/other
Format text/markdown; application/zip
Discipline Materials Science and Engineering